Hydrogen production through the aqueous phase reforming of ethylene glycol over supported Pt-based bimetallic catalysts

Kim, Ho Dong; Park, Hyun Ju; Kim, Tae Wan; Jeong, Kwang Eun; Chae, Ho Jeong; Jeong, Soon Yong; Lee, Chang Ha; Kim, Chul Ung

doi:10.1016/j.ijhydene.2012.02.160

Cited by 43 publications

(32 citation statements)

References 32 publications

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“…Similar to the case of CMK-3 based catalysts, 50,51 the narrow pore size distribution inside carbide-derived carbons as well as regular structure and high surface area of carbons might facilitate APR thus resulting in enhanced TOF H2 and TOF alk . Furthermore, the interactions between Pt and carbide-derived support might enhance the catalytic performance.…”

Section: Catalysis Science and Technology Papermentioning

confidence: 93%

Aqueous-phase reforming of xylitol over Pt/C and Pt/TiC-CDC catalysts: catalyst characterization and catalytic performance

Кирилин

Hasse

Tokarev

et al. 2014

Catal. Sci. Technol.

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aThe aqueous phase reforming (APR) of xylitol was studied over five Pt/C catalysts. The correlation between physico-chemical properties of the catalysts and catalytic performance was established. The Pt/C catalysts have different textural properties as well as different mean Pt cluster sizes and surface acidity. The average Pt cluster size was investigated by means of CO chemisorption as well as by TEM.The reaction was found to be structure sensitive and TOF linearly increases with increasing average Pt cluster size in the studied domain. The catalysts which possess higher surface acidity favoured higher rates of hydrocarbon production. On the contrary the Pt/C materials with lower acidities generated hydrogen with high selectivity and TOF.

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Section: Catalysis Science and Technology Papermentioning

confidence: 93%

Aqueous-phase reforming of xylitol over Pt/C and Pt/TiC-CDC catalysts: catalyst characterization and catalytic performance

Кирилин

Hasse

Tokarev

et al. 2014

Catal. Sci. Technol.

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“…On the other hand, the strong interaction between Pt and Mn formed PteMn alloys. The addition of Mn considerably enhanced H 2 yield in comparison with monometallic Pt catalyst and other bimetallic combinations [98].…”

Section: Hydrogen Formationmentioning

confidence: 94%

A review of catalytic aqueous-phase reforming of oxygenated hydrocarbons derived from biorefinery water fractions

Coronado

Stekrova

Reinikainen

et al. 2016

International Journal of Hydrogen Energy

135

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“…Kim et al [68] used Pt bimetallic catalysts with other metals on different supports, with WHSV of 2.0 h −1 at 250˚C, and 45 atm. Pt-Mn bimetallic catalysts on CNK-3 support had the highest activity of hydrogen production among all monometallic catalysts, reaching TOF H2 of 180 min −1 at peaks.…”

Section: Ethylene Glycolmentioning

confidence: 99%

Renewable Hydrogen Produced from Different Renewable Feedstock by Aqueous-Phase Reforming Process

Wei¹,

Lei²,

Liu³

et al. 2014

JSBS

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Aqueous phase reforming (APR) of biomass derived feedstock producing hydrogen was reviewed. The APR process was discussed based on different feedstock categories such as sugars, polyols and ethanol. The mechanism of APR was analyzed referring to different structures of feedstock. The reaction pathways of APR were investigated. The usage of catalysts should be judged by feedstock on the requirement including C-C bond cleavage, water-gas shift (WGS) reaction, and catalyst maintenance. The prospects were concluded based on the recent works from bimetallic catalysts and high efficient supports. Examples of significant challenges of reducing catalyst cost and increasing catalyst stability have been discussed. The modification and utilization of alkane selectivity of APR processes for liquid fuel production was also investigated.

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Hydrogen production through the aqueous phase reforming of ethylene glycol over supported Pt-based bimetallic catalysts

Cited by 43 publications

References 32 publications

Aqueous-phase reforming of xylitol over Pt/C and Pt/TiC-CDC catalysts: catalyst characterization and catalytic performance

Aqueous-phase reforming of xylitol over Pt/C and Pt/TiC-CDC catalysts: catalyst characterization and catalytic performance

A review of catalytic aqueous-phase reforming of oxygenated hydrocarbons derived from biorefinery water fractions

Renewable Hydrogen Produced from Different Renewable Feedstock by Aqueous-Phase Reforming Process

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