Hydrogen‐Bond‐Based Polymer‐Ammonium Intermediates Induced Buried Interface Engineering for High‐Performance Inverted Perovskite Solar Cells
Xin Zhao,
Ruixi Luo,
Chen Yu
et al.
Abstract:Perovskite interfaces where defects enrich are pivotal for both device efficiency and stability. Herein, a high‐molecular‐weight polyvinyl pyrrolidone (PVP) is proposed as a robust multi‐functional interlayer to engineer the buried interface. Besides the well‐known defect passivation, perovskite crystallization is intriguingly modulated via the formation of hydrogen‐bond‐based polymer‐ammonium intermediates (e.g., PVP‐FA+ or PVP‐MA+, where MA and FA are methylamine and formamidine, respectively). The interacti… Show more
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