2019
DOI: 10.1021/acs.jpclett.9b02249
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Humidity-Driven Soft Actuator Built up Layer-by-Layer and Theoretical Insight into Its Mechanism of Energy Conversion

Abstract: An improved protocol is proposed for preparation of a humiditysensitive soft actuator through the layer-by-layer assembling of weight-ratio-variable composites of sodium alginate (SA) and poly(vinyl alcohol) (PVA) into laminated structures. The design induces nonuniform hygroscopicity in the thickness direction and gives rise to strong interfacial interaction between layers, making the actuator have directional motility. A mathematical model reveals that the directional motion is driven by the chemical potenti… Show more

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Cited by 31 publications
(29 citation statements)
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“…Using this actuator, they achieved an energy conversion efficiency of 81.2% at 25 °C. [157] Besides the bilayer structures, the aligned microstructures of the plants have a significant role in their actuation and response time. Cellulose materials (cellulose nanofibers, cellulose nanocrystals, bacterial cellulose) are super hydrophilic nanostructures that can enhance response time (Figure 9D,E).…”
Section: Anisotropic Swellingmentioning
confidence: 99%
“…Using this actuator, they achieved an energy conversion efficiency of 81.2% at 25 °C. [157] Besides the bilayer structures, the aligned microstructures of the plants have a significant role in their actuation and response time. Cellulose materials (cellulose nanofibers, cellulose nanocrystals, bacterial cellulose) are super hydrophilic nanostructures that can enhance response time (Figure 9D,E).…”
Section: Anisotropic Swellingmentioning
confidence: 99%
“…A typical actuator, also known as artificial muscle, is the work horse of soft robots. [ 34 ] It typically needs external stimuli, such as water, [ 35 , 36 , 37 , 38 , 39 , 40 , 41 , 42 , 43 , 44 , 45 ] pH, [ 46 , 47 , 48 , 49 , 50 ] heat, [ 47 , 51 , 52 , 53 , 54 , 55 , 56 , 57 ] light, [ 58 , 59 , 60 , 61 , 62 , 63 , 64 , 65 ] electricity, [ 53 , 66 , 67 , 68 , 69 , 70 , 71 ] and magnetic field to perform. [ 27 , 72 , 73 , 74 , 75 ] In recent years, soft actuators can be classified based on materials as elastomeric pneumatic actuator (PA), hydrogel actuator (HA), bio‐hybrid actuator (BHA), actuators made of DE, twisted and coiled yarns (TCY), SMA, liquid crystal elastomers (LCE), and ionic polymer‐metal composites (IPMC).…”
Section: Biomimetic Functions and Potential Applicationsmentioning
confidence: 99%
“…[1][2][3][4][5][6][7][8] This energy transformation can be achieved by the reversible deformation of materials (e.g., contraction, expansion, rotation, bending, twisting, and curling) under external stimuli such as electrical fields, temperature, light, pH, vapor, and pressure. [9][10][11][12] At present, most mechanically responsive materials are based on polymeric materials, including organic polymers, hydrogels, and liquid crystal elastomers, [13][14][15][16][17] while relatively less focus has been put on molecular crystals that possess precisely determined structures with ordered molecular packing. Molecular crystals exhibit considerable advantages as smart materials that can surpass traditional polymeric materials, such as rapid response, faster relaxation recovery, and a higher Young's modulus.…”
Section: Introductionmentioning
confidence: 99%