CP -violation in the quark sector has been well established over the last decade, but has not been observed in the lepton sector. We search for CP -violating decay processes in positronium, using the angular correlation of ( S · k1)( S · k1 × k2), where S is the the positronium spin and k1, k2 are the directions of the positronium decay photons. To a sensitivity of 2.2 × 10 −3 , no CP -violation has been found, which is at the level of the CP -violation amplitude in the K meson. A 90% confidence interval of the CP -violation parameter (CCP ) was determined to be −0.0023 < CCP < 0.0049. This result is a factor 7 more strict than that of the previous experiment.The material state of the universe results only because of its matter-antimatter asymmetry. To understand the origin of this asymmetry is one of particle physics' most urgent goals. One cause could be the CPviolation (charge conjugation and parity) in the quark sector, which was found both in the K [1] and B [2] mesons. The CP -violating processes in B mesons have been measured precisely [3] using its various decay processes at KEKB and PEP-II and they can be well described with the Kobayashi-Maskawa theory [4]. While understanding the origin of CP -violation in the quark sector is a great achievement, the resulting asymmetry may be too small to result in the amount of matter in the Universe [5]. All CP -violating observables in the Standard Model are proportional to the Jarlskog invariance, J= s 2 1 s 2 s 3 c 1 c 2 c 3 sin(δ) ∼ 3 × 10 −5 , where c i are s i are the mixing angles in the KM matrix, and δ is the CP -violating phase. The CP -violating observables are also suppressed by the Higgs vacuum expectation value, 1/v 12 , since non-equilibrium can occur in the electroweak phase transition in the Standard Model. It seems that these violations alone are too small to accout for the observed baryons in the universe. A new source of CP -violation or a new mechanism is necessary, and CPviolation in the lepton sector [6] is a good candidate. Leptonic CP -violation has not yet been observed despite many studies at various neutrino factories [7].Positronium (Ps) is a neutral system comprising an electron and a positron and is the analogue of the neutral meson. If CP is violated in the lepton sector, such neutral systems (e.g. Ps, muonium) are good test candidates since the admixture of opposite CP eigenstates will occur. The search for CP -violation in Ps has been performed previously and no CP violation was found at the 1.5% level of uncertainty [9].If CP -symmetry is not conserved in Ps, the decay rate of the triplet Ps (o-Ps) is dependent on the CP -violating term. The number of o-Ps decay events would be expressed as (1) where S is the spin of the o-Ps, k i is the direction of the i-th energetic γ-ray from the decay (| k i |=1), and τ is the lifetime of o-Ps. C CP is the amplitude of the CP -violation. The Standard Model prediction for C CP is of the order of 10 −10 [10]. This is due to photonphoton interactions in the final state. Another exotic decay cont...