2011
DOI: 10.1103/physrevlett.106.127401
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Hot-Electron-Driven Enhancement of Spin-Lattice Coupling in Gd and Tb4fFerromagnets Observed by Femtosecond X-Ray Magnetic Circular Dichroism

Abstract: Femtosecond x-ray magnetic circular dichroism was used to study the time-dependent magnetic moment of 4f electrons in the ferromagnets Gd and Tb, which are known for their different spin-lattice coupling. We observe a two-step demagnetization with an ultrafast demagnetization time of 750 fs identical for both systems and slower times which differ sizeably with 40 ps for Gd and 8 ps for Tb. We conclude that spin-lattice coupling in the electronically excited state is enhanced up to 50 times compared to equilibr… Show more

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Cited by 169 publications
(209 citation statements)
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References 33 publications
(47 reference statements)
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“…Even though the two sublattices are exchange coupled, they still demagnetize at different rates as in their pure ferromagnetic form 17,18 . This non-equivalence of the sublattices is essential for the reversal, requiring different rates of demagnetization in each sublattice.…”
Section: Discussionmentioning
confidence: 99%
“…Even though the two sublattices are exchange coupled, they still demagnetize at different rates as in their pure ferromagnetic form 17,18 . This non-equivalence of the sublattices is essential for the reversal, requiring different rates of demagnetization in each sublattice.…”
Section: Discussionmentioning
confidence: 99%
“…One indication of this effect has been found by Erekhinsky et al [45] in a transport experiment. Another indication is the fact, that for gadolinium, the surface demagnetizes within <100 fs (measured by second harmonic magneto-optical Kerr effect [46]), whereas the bulk needs approx. 1 ps [47].…”
Section: The Role Of the Interface For The Demagnetizationmentioning
confidence: 99%
“…13,[37][38][39][40][41][42] In ferrimagnets, there is a large interest on demagnetization rates of each species, following the use of X-ray magnetic circular dichroism 5 to monitor the sub-picosecond dynamics of each sublattice magnetization individually. 4 Thermal effects dominate the magnetization dynamics during the heating produced by the laser.…”
Section: Estimation Of the Temperature Dependent Magnetization Relmentioning
confidence: 99%