In this paper, a bicharacteristic waveguide (BW) is proposed for fundamental-mode phase-matched second harmonic generation (SHG) from mid-infrared (MIR) to near-infrared (NIR). The required phase matching condition (PMC) is satisfied between the fundamental plasmonic mode at 3100 nm and the photonic mode at 1550 nm. With 1 W pump power, the SHG conversion efficiency of 4.173% can be obtained in 90.3 μm length waveguide. Moreover, the SHG conversion can be enhanced by using a microring resonator (MRR). By optimizing the MRR, the SHG conversion efficiency is increased to 8.30%. The proposed waveguide can also provide a promising platform for upconversion detection. By using an on-chip cascaded configuration, a gas sensor with the capability of MIR absorption and NIR detection is proposed. It is found that the detection limit (DL) can reach 1.04 nmol/L with 100 mW pump power, which shows significant enhancement compared with direct MIR absorption and detection.
IntroductionSecond-order nonlinear optical processes such as second harmonic generation (SHG) have significant applications in various fields e.g. all-optical signal processing [1], wavelength conversion [2], optical switch [3], etc. Benefiting from the planar integrated geometric structure and tight mode profile, optical waveguides provide a potential platform for efficient SHG [4]. Over the last few decades, plasmonic waveguides have attracted great attention in nonlinear photonics due to their extraordinary abilities to break through the traditional optical diffraction limits [5]. Recently, some plasmonic SHG waveguides have been extensively studied, such as the waveguide combined a second-order nonlinear material lithium niobate (LiNbO 3 ) and a plasmonic structure [6][7][8]. Furthermore, the conversion efficiency can be significantly improved by employing polymer material with much higher second-order nonlinearity [9,10].Phase matching conditions (PMCs) which ensure the continuous power transfer from pump to harmonic are vital to realize efficient SHG process. Currently, the frequently utilized PMC techniques are based on quasi-phase matching (QPM) or intermodal-phase matching (IMPM) [11][12][13][14]. However, the QPM usually relies on the iron exchange technology or grating structure which can complicate the fabrication process. For IMPM, the generated harmonic is in the form of higher-order mode (HOM) which is difficult for post manipulation. Particularly, it is inferior for the application such as photon pair generation since an additional mode convertor is required to produce the target pump mode. Therefore, realizing the PMC between fundamental