Highly efficient deep-blue organic light-emitting diodes (OLEDs) based on hot-exciton materials with multiple triplet exciton conversion channels
Mizhen Sun,
Chenglin Ma,
Lizhi Chu
et al.
Abstract:High-energy triplet exciton conversion, high exciton utilization efficiency and high device efficiency were achieved through multiple hot-exciton conversion channels.
“…For 2(3ph)-phCz, another introduction of 3ph group provides a larger steric hindrance, which leads to 2(3ph)-phCz possessing relatively loose molecular packing compared to 3ph-phCz. 36 As for 2(3phCN)-phCz, the additional unit (3phCN) provided a large steric hindrance to endow 2(3phCN)-phCz with a relatively loose molecular packing, which easily leads to configurational relaxation of the excited state to enhance the nonradiative process and lowers the PLQY in films.…”
The hybrid local and charge transfer (HLCT) molecules have garnered considerable attention for their potential in the full utilization of excitons and efficient blue luminescence. Here, we proposed a molecular...
“…For 2(3ph)-phCz, another introduction of 3ph group provides a larger steric hindrance, which leads to 2(3ph)-phCz possessing relatively loose molecular packing compared to 3ph-phCz. 36 As for 2(3phCN)-phCz, the additional unit (3phCN) provided a large steric hindrance to endow 2(3phCN)-phCz with a relatively loose molecular packing, which easily leads to configurational relaxation of the excited state to enhance the nonradiative process and lowers the PLQY in films.…”
The hybrid local and charge transfer (HLCT) molecules have garnered considerable attention for their potential in the full utilization of excitons and efficient blue luminescence. Here, we proposed a molecular...
“…25 By modifying anthracene with various donor (D) and/or acceptor (A) groups, the excited state properties can be tuned to enhance the hRISC process. 26–29 However, most anthracene-based hot exciton emitters have difficulty in achieving a high EQE in deep-blue light emission, and they usually have a relatively large full width at half maximum (FWHM) resulting in low color purity.…”
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