4397wileyonlinelibrary.com circuit simplicity when interfacing to standard AC power sources. However, as with all ultrathin or organic lighting approaches, a widely sought property of the AC-OEL is fl exibility.The concept of low-cost, fl exible, higheffi ciency light sources based on organic solid-state lighting devices is already well established. [14][15][16][17][18][19] Indeed, both standard organic light emitting diodes (OLEDs) as well as AC-OELs have demonstrated brightness and effi ciency numbers of commercial interest. However, the slow transition from state-of-the-art laboratory research to a modern manufacturing environment should somehow indicate the magnitude of the challenges faced by the technologies to meet with robust utilization in the consumer world. [ 20 ] Two key problems that developers are facing are addressed in this work.The fi rst is how to achieve extremely high-power effi ciencies in lighting devices when internal quantum effi ciencies are already reaching levels approaching 100% (both the spin-symmetric and antisymmetric molecular excitations are fully used for photon emission. [21][22][23][24][25] In any organic EL device, there are many energy loss mechanisms from carrier transport to multiple nonradiative processes that convert singlet and triplet excitations into the ground state. [21][22][23][24] Among these mechanisms, an important problem in OLEDs is direct injection of hot carriers, which form bound electron-hole pairs or excitons after tunneling through energy barriers at multiple interfaces. [26][27][28][29] These hot carriers exceed the energy gap of the emitting material, so the excess energy is wasted thermally, giving rise to a lower power effi ciency. The reduction of the carrier injection barrier by decreasing the difference between adjacent energy levels (highest occupied molecular orbital (HOMO) or lowest unoccupied molecular orbital (LUMO)) is now a common method to optimize the efficiency of OLEDs. [30][31][32][33][34] However, as in the case with most technology demonstrators, what works best in the lab is diffi cult to implement in commercial settings, so placing Li or Ca at the metal interface is undesirable.In the case of capacitively coupled AC-OEL devices, as described here, the large induced polarization currents effectively control the rate and energy of carrier "injection." While power effi ciencies as high as 29.3 lm W −1 at 20 500 cd m −2 have been reported in green phosphorescent AC-OEL devices, it has In this work, the application of an aluminum (Al)/multiwall carbon nanotube (MWCNT)/Al, multilayered electrode to fl exible, high-effi ciency, alternating current driven organic electroluminescent devices (AC-OEL), is reported. The electrode is fabricated by sandwiching a spray-cast nanonetwork fi lm of MWCNTs between two evaporated layers of Al. The resulting composite fi lm facilitates a uniform charge distribution across a robust crack-free electrode under various bending angles. It is demonstrated that these composite electrodes stabilize the power eff...