1998
DOI: 10.1063/1.122077
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High temperature excitonic stimulated emission from ZnO epitaxial layers

Abstract: The emission spectrum of high quality ZnO epilayers is studied from room temperature up to 550 K. At room temperature and low excitation power a single emission peak is observed which may be identified with the free exciton from its peak energy and dependence on temperature. However, when excitation intensities exceed 400 kW cm−2 a sharp peak emerges at lower energy which we attribute to exciton-exciton scattering. At higher excitation intensities (>800 kW cm−2) a second stimulated emission peak emerges… Show more

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Cited by 783 publications
(390 citation statements)
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“…The similarity of the ZnO-layer CL spectrum and the LED EL spectrum, and the thermostability of the emission and very large exciton binding energy of ZnO ͑ϳ60 meV͒, suggest that the UV emission of the n-ZnO/p-AlGaN LED is mainly excitonic in nature. In earlier reports, Bagnall et al 13 observed stimulated excitonic emission at relatively high temperatures, up to 550 K. However, other radiative mechanisms, such as donor-acceptor, donor-hole, and acceptor-electron transitions can also take place and contribute to this EL NBE emission.…”
mentioning
confidence: 99%
“…The similarity of the ZnO-layer CL spectrum and the LED EL spectrum, and the thermostability of the emission and very large exciton binding energy of ZnO ͑ϳ60 meV͒, suggest that the UV emission of the n-ZnO/p-AlGaN LED is mainly excitonic in nature. In earlier reports, Bagnall et al 13 observed stimulated excitonic emission at relatively high temperatures, up to 550 K. However, other radiative mechanisms, such as donor-acceptor, donor-hole, and acceptor-electron transitions can also take place and contribute to this EL NBE emission.…”
mentioning
confidence: 99%
“…For the past few years, the lasing characteristics in ZnO films [1,2] and powders [3] have been widely investigated. These studies, along with the discovery and understanding of single nanowire lasers [4], have led to a number of investigations pertaining to the growth and characterization of ZnO microcavity lasers [5,6].…”
Section: Introductionmentioning
confidence: 99%
“…However, there is a revival of interest in the materials because of their potential applications in optoelectronic devices employing excitonic effects in the short wavelength range, due to their large exciton binding energy, etc. Among them, ZnO has rapidly emerged as a promising analog to GaN, after the demonstration of the excitonic emission at elevated temperatures up to 550 K (Bagnall et al, 1998). Despite considerable success in optimizing the growth conditions and structural quality such as the fabrication of blue photoemitters (Tsukazaki et al, 2005), ZnO epilayers still contain a number of defects.…”
Section: Dislocations In Wide Gap Semiconductorsmentioning
confidence: 99%