We have performed the photoemission spectroscopy of the bilayered manganese oxides La 2−2x Sr 1+2x Mn 2 O 7 (x = 0.38, 0.40) with the photon energies (hν) of 640-700 eV and 8150 eV. The difference between the surface and the bulk electronic structures is revealed from the polar-angle dependence of the Sr 3d core level and the valence band spectra with hν = 700 eV. Moreover, we have reconfirmed that the spectral weight at the Fermi level is suppressed even in the bulk electronic states by means of the valence band spectra obtained by the Mn 2p-3d resonant photoemission with hν ∼ 643eV and by the hard-X-ray photoemission spectroscopy with 8175eV photons.