2012
DOI: 10.1209/0295-5075/98/24001
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High-order optical nonlinearity at low light levels

Abstract: We observe a nonlinear optical process in a gas of cold atoms that simultaneously displays the largest reported fifth-order nonlinear susceptibility χ (5) = 1.9×10 −12 (m/V) 4 and high transparency.The nonlinearity results from the simultaneous cooling and crystallization of the gas, and gives rise to efficient Bragg scattering in the form of six-wave-mixing at low-light-levels. For large atom-photon coupling strengths, the back-action of the scattered fields influences the light-matter dynamics. This system m… Show more

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Cited by 33 publications
(24 citation statements)
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“…We observe that decreasing |∆| and increasing OD result in smaller values of I thresh , since these changes enhance the lightmatter coupling strength [19,21]. The measured values of I thresh agree well with the model developed in Refs.…”
supporting
confidence: 89%
See 1 more Smart Citation
“…We observe that decreasing |∆| and increasing OD result in smaller values of I thresh , since these changes enhance the lightmatter coupling strength [19,21]. The measured values of I thresh agree well with the model developed in Refs.…”
supporting
confidence: 89%
“…The measured values of I thresh agree well with the model developed in Refs. [19] and [21] to describe the light-matter interaction in our system, where we take I thresh as the value of I p for which the gain becomes infinite. The lowest threshold we measure is I thresh = 1.1 ± 0.25 mW/cm 2 , which occurs for ∆/Γ = −3 and OD = 20 ± 1 and is comparable to the threshold intensity observed for a Bose-Einstein condensate [8].…”
mentioning
confidence: 99%
“…In recent years, self-organizing instabilities due to the opto-mechanical coupling of light and cold [9][10][11][12][13][14] and ultracold [15,16] atoms have attracted remarkable interest. In many of these schemes a pump beam is scattered by the gas into an externally imposed mode (often selected by a cavity).…”
mentioning
confidence: 99%
“…When coupling the dynamics of light and the centre-of-mass degrees of freedom of laser-cooled atoms, the dynamics becomes nonlinear and, above a critical value for the energy injected into the system, a transition is observed from a spatially homogeneous state to a state displaying some form of long-range order. This can be obtained in various configurations: transversally pumped cavities [1] where collective dynamics and self-organization in cold [2,3] and ultracold [4] gases have been investigated; collective atomic recoil lasing (CARL) where the spontaneous generation of a back-scattered beam within a monodirectional cavity is self-sustained by atomic bunching in the resulting optical potential [5][6][7]; in a counter-propagating geometry super-radiance and highorder nonlinearities stemming from atomic bunching have been studied [8][9][10] a continuous translational symmetry in the presence of a strong viscous damping was investigated for both cavity [11,12] and counter-propagating [10,13,14] geometries, whereas a single-mirror geometry in the absence of damping was the focus of recent theoretical [15] and experimental [16] research. The distinguishing feature of these studies is that the spatial scale of the emerging spatial structure is self-selected, so that the spontaneous breaking of two continuous symmetries is observed (rotations and translations in the plane).…”
Section: Introductionmentioning
confidence: 99%