“…Carbon-based materials have been predominantly used for EDLCs, such as mesoporous carbon, activated carbon, carbon aerogel, carbon nanotubes and graphene [14].Transition metals oxides (such as MnO2, NiO, Co3O4, RuO2), chalcogenides (Co9S8, Ni3S2, etc), hydroxides [Co(OH)2, Ni(OH) 2, etc] and conducting polymers (polypyrrole, polyaniline, etc) have been intensively studied as electrode materials for pseudocapacitors [10,[15][16][17]. Among them, ternary nickel cobaltite sulfide (NiCo2S4 or CoNi2S4, denoted as NCS) have been recognized as one of the most promising candidates for electrode materials due to some special characters, such as high electrical conductivity, high electrochemical activity, environmental friendliness and low cost [18,19].…”