2023
DOI: 10.1002/advs.202204120
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Heat‐Driven Iontronic Nanotransistors

Abstract: Thermoelectric polyelectrolytes are emerging as ideal material platform for self-powered bio-compatible electronic devices and sensors. However, despite the nanoscale nature of the ionic thermodiffusion processes underlying thermoelectric efficiency boost in polyelectrolytes, to date no evidence for direct probing of ionic diffusion on its relevant length and time scale has been reported. This gap is bridged by developing heat-driven hybrid nanotransistors based on InAs nanowires embedded in thermally biased N… Show more

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Cited by 6 publications
(4 citation statements)
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“…[EMIM + ] [TFSI − ] is commonly used as an electrolyte for ion gate experiments [16,18,32]. It is liquid at room temperature and freezes below 220 K. It has an electrochemical window of 4.7 eV, with an anodic limit of 2.6 eV and a cathodic limit of −2.1 eV [33,34].…”
Section: Resultsmentioning
confidence: 99%
See 1 more Smart Citation
“…[EMIM + ] [TFSI − ] is commonly used as an electrolyte for ion gate experiments [16,18,32]. It is liquid at room temperature and freezes below 220 K. It has an electrochemical window of 4.7 eV, with an anodic limit of 2.6 eV and a cathodic limit of −2.1 eV [33,34].…”
Section: Resultsmentioning
confidence: 99%
“…In the past few years, the combination of the properties of InAs NWs and the exceptional effectiveness of ion gating has begun to demonstrate its potential [11,17,18]. InAs NWs possess interesting properties, such as the high aspect ratio, and strong spin-orbit coupling [19], which make them promising for a broad range of applications including nanoelectronics [20,21], optoelectronics [22], spintronics [19], sensing [23,24] and quantum technologies [25][26][27].…”
Section: Introductionmentioning
confidence: 99%
“…In this context, TMDs provide an ideal material platform to be employed in integrated photonic devices, owing to their flexibility in terms of material properties [116] and access to reversible tuning of their electrical properties by exploiting ionic liquid gating-a non conventional gating technique which has been proven to outperform conventional gating techniques [117,118]. Figure 5 shows representative examples of the integration of TMDs on silicon photonic platforms.…”
Section: Two-dimensional Materials Integration In Integrated Photonic...mentioning
confidence: 99%
“…In this frame, nanowires are given particular attention, due to their large aspect ratio allowing for reduced thermal conductivity with respect to the bulk counterpart, and thanks to the reliability of device fabrication protocols and control methods. Leveraging on unique combinations of newly engineered nanowire heterostructures, advanced nanofabrication techniques and innovative control strategies , such as electrolyte gating, seminal results were recently achieved including the giant reduction of thermal conductivity in twinning superlattice InAsSb nanowires [8], and the demonstration of heat-driven transistors at the nanoscale [9].…”
mentioning
confidence: 99%