Piezoresistive
pressure sensors have garnered significant attention
because of their wide applications in automobiles, intelligent buildings,
and biomedicine. For in vivo testing, the size of pressure sensors
is a vital factor to monitor the pressure of specific portions of
a human body. Therefore, the primary focus of this study is to miniaturize
piezoresistive pressure sensors with graphene oxide (GO)-incorporated
poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS)
composite films on a flexible substrate for biomedical applications.
Prior to the fabrication of pressure sensors, a comprehensive material
analysis was applied to identify the horizontal placement of GO flakes
within the PEDOT:PSS copolymers, revealing a reduction in variable
range hopping distance and an enhancement in carrier mobility. For
devices scaled to 0.2 cm, the sensitivity of PEDOT:PSS pressure sensors
was conspicuously decreased owing to the late response, which can
be effectively solved by GO incorporation. Using technology computer-aided
design simulations, the current crowded at the PEDOT:PSS film surface
and in the vicinity of an indium–tin–oxide electrode
corner was found to be responsible for the changes in piezoresistive
behaviors of the scaled devices. The miniaturized flexible piezoresistive
pressure sensors with PEDOT:PSS/GO composite films are capable of
monitoring the brain pressure of intracranial surgery of a rat and
discerning different styles of music for a potential application in
hearing aids.