We report the experimental realization and characterization of one 60-mode copy, and of two 30-mode copies, of a dual-rail quantum-wire cluster state in the quantum optical frequency comb of a bimodally pumped optical parametric oscillator. This is the largest entangled system ever created whose subsystems are all available simultaneously. The entanglement proceeds from the coherent concatenation of a multitude of EPR pairs by a single beam splitter, a procedure which is also a building block for the realization of hypercubic-lattice cluster states for universal quantum computing.PACS numbers: 03.65. Ud,03.67.Bg,42.50.Dv,03.67.Mn, 42.50.Ex , 42.65.Yj Introduction.-Initially identified by Einstein, Podolsky, and Rosen (EPR) [1] as central to testing the completeness of quantum mechanics, entanglement is also crucial to exponential speedups of quantum computing [2][3][4][5]. In the race to build a practical quantum computer [6], the ability to create very large quantum registers and entangle them is paramount, along with the ability to address the issue of decoherence. The study of large-scale entanglement-i.e., multipartite entanglement between numerous subsystems-is in itself an intriguing topic at the forefront of current research, as such systems have yet to be studied in laboratories.Until recently, the largest entangled state of any sort involved 14 trapped ions [7]. Quantum optical systems, which suffer less from decoherence but are harder to entangle, have shown progress, with photon-based, discrete-variable implementations of a 4-qubit "compiled," nonscalable version of Shor's algorithm [8, 9], including in an integrated optics platform [10], 4-qubit blind quantum computing [11], and 8-qubit topological quantum error correction [12].With particular regard to scalability, the field-based, continuous-variable (CV) flavor of quantum optics has high potential [13][14][15][16][17], in particular by enabling "top down," rather than "bottom up," entangling approaches of quantum field modes. It is also important to note the relevance of continuous variables to universal quantum computing, with the recent discovery of a fault tolerance threshold for quantum computing with CV cluster states and nonGaussian error correction [18].In 2011, 15 independent 4-mode cluster states were generated simultaneously over 60 modes of the quantum optical frequency comb (QOFC) of a single optical parametric oscillator (OPO) [19]. In 2013, 10-mode entanglement was observed in a synchronously pumped OPO [20], and 10,000 modes were sequentially entangled into a dual-rail cluster state [21] following a time-domain protocol [22, 23] in which the modes are emitted in pairs and detected in turn, with only a few modes accessible