Abstract:We demonstrate scalable terahertz (THz) generation by focusing terawatt, two-color laser pulses in air with a cylindrical lens. This focusing geometry creates a two-dimensional air plasma sheet, which yields two diverging THz lobe profiles in the far field. This setup can avoid plasma-induced laser defocusing and subsequent THz saturation, previously observed with spherical lens focusing of high-power laser pulses. By expanding the plasma source into a two-dimensional sheet, cylindrical focusing can lead to sc… Show more
“…Currently, the most powerful table-top THz sources are based on either optical rectification in electro-optic crystals [17][18][19] or twocolor filamentation in gases and liquids [20][21][22][23][24] . With optical rectification THz pulses with energy up to 0.9 mJ 18 and THz conversion efficiency (ratio of generated THz energy to the input laser pulse energy) up to 3.7% 25 were generated.…”
mentioning
confidence: 99%
“…Also, THz pulses generated by optical rectification are long (several picoseconds) and their spectra are narrow (below 5 THz). In turn, two-color filamentation of near infrared laser pulses offers less energetic THz pulses (up to 30 μJ in gases 22 and up to 80 μJ in liquids 24 ) with a lower THz conversion efficiency (~0.01%). Nevertheless, since the gas or liquid media recover in-between laser shots, there is no issue with the optical damage threshold.…”
Extreme nonlinear interactions of THz electromagnetic fields with matter are the next frontier in nonlinear optics. However, reaching this frontier in free space is limited by the existing lack of appropriate powerful THz sources. Here, we experimentally demonstrate that two-color filamentation of femtosecond mid-infrared laser pulses at 3.9 μm allows one to generate ultrashort sub-cycle THz pulses with sub-milijoule energy and THz conversion efficiency of 2.36%, resulting in THz field amplitudes above 100 MV cm −1. Our numerical simulations predict that the observed THz yield can be significantly upscaled by further optimizing the experimental setup. Finally, in order to demonstrate the strength of our THz source, we show that the generated THz pulses are powerful enough to induce nonlinear cross-phase modulation in electro-optic crystals. Our work paves the way toward free space extreme nonlinear THz optics using affordable table-top laser systems.
“…Currently, the most powerful table-top THz sources are based on either optical rectification in electro-optic crystals [17][18][19] or twocolor filamentation in gases and liquids [20][21][22][23][24] . With optical rectification THz pulses with energy up to 0.9 mJ 18 and THz conversion efficiency (ratio of generated THz energy to the input laser pulse energy) up to 3.7% 25 were generated.…”
mentioning
confidence: 99%
“…Also, THz pulses generated by optical rectification are long (several picoseconds) and their spectra are narrow (below 5 THz). In turn, two-color filamentation of near infrared laser pulses offers less energetic THz pulses (up to 30 μJ in gases 22 and up to 80 μJ in liquids 24 ) with a lower THz conversion efficiency (~0.01%). Nevertheless, since the gas or liquid media recover in-between laser shots, there is no issue with the optical damage threshold.…”
Extreme nonlinear interactions of THz electromagnetic fields with matter are the next frontier in nonlinear optics. However, reaching this frontier in free space is limited by the existing lack of appropriate powerful THz sources. Here, we experimentally demonstrate that two-color filamentation of femtosecond mid-infrared laser pulses at 3.9 μm allows one to generate ultrashort sub-cycle THz pulses with sub-milijoule energy and THz conversion efficiency of 2.36%, resulting in THz field amplitudes above 100 MV cm −1. Our numerical simulations predict that the observed THz yield can be significantly upscaled by further optimizing the experimental setup. Finally, in order to demonstrate the strength of our THz source, we show that the generated THz pulses are powerful enough to induce nonlinear cross-phase modulation in electro-optic crystals. Our work paves the way toward free space extreme nonlinear THz optics using affordable table-top laser systems.
“…It is worth noting the new variety of materials on the basis of which the efficient sources of terahertz radiation are being created [10,11]. The most popular mechanism is terahertz generation via filamentation in gases with one or two-color optical excitation due to the possibility to control output radiation by the pump laser parameters [12][13][14][15]. Using two-color filamentation, maximum efficiency is around 0.01% [16].…”
Polar liquids are strong absorbers of electromagnetic waves in the terahertz range, therefore, historically such liquids have not been considered as good candidates for terahertz sources. However, flowing liquid medium has explicit advantages, such as a higher damage threshold compared to solid-state sources and more efficient ionization process compared to gases. Here we report systematic study of efficient generation of terahertz radiation in flat liquid jets under sub-picosecond single-color optical excitation. We demonstrate how medium parameters such as molecular density, ionization energy and linear absorption contribute to the terahertz emission from the flat liquid jets. Our simulation and experimental measurements reveal that the terahertz energy has quasi-quadratic dependence on the optical excitation pulse energy. Moreover, the optimal pump pulse duration, which depends on the thickness of the jet is theoretically predicted and experimentally confirmed. The obtained optical-to-terahertz energy conversion efficiency is more than 0.05%. It is comparable to the commonly used optical rectification in most of electro-optical crystals and two-color air filamentation. These results, significantly advancing prior research, can be successfully applied to create a new alternative source of terahertz radiation.
“…Recently, Xie et al [3] delivered frequency doubled beams (2ω) time delayed with respect to the original pulse beam (ω), and Peng et al [8] also used an adjustable aperture to tailor the Gaussian beam to obtain enhanced THz radiation. Another study [9] showed that the energy conversion efficiency of the second harmonic method can be improved using a cylindrical lens. This changes the focal spot and the shape of the filament, improving the structure of the photocurrent within the filament and controllability of the radiation pattern and generation efficiency.…”
We apply active feedback optimization methods to pyroelectric measurements of a THz signal generated by four wave mixing in air using 1 mJ to 12 mJ, 35 fs laser pulses operating at 12 kHz repetition rate. A genetic algorithm, using the THz signal as a figure of merit, determines the voltage settings to a deformable mirror and results in up to a 6 fold improvement in the THz signal compared with settings optimized for the best focus. It is possible to optimize for different THz generation processes using this technique.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.