The laser system PALS, as a driver of a broad-beam ion source, delivered deuterons which generated neutrons with energies higher than 14 MeV through the 7 Li(d, n) 8 Be reaction. Deuterons with sub-MeV energy were accelerated from the front surface of a massive CD 2 target in the backward direction with respect to the laser beam vector. Simultaneously, neutrons were emitted from the primary CD 2 target and a secondary LiF catcher. The total maximum measured neutron yield from 2 D(d, n) 3 He, 7 Li(d, n) 8 Be, 12 C(d, n) 13 N reactions was ∼3.5(±0.5) × 10 8 neutrons/shot.