Ga-Induced p–d Orbital Hybridization in CoFe LDH for Boosted Oxygen Evolution Electrocatalysis
Qie Fang,
Lijin Wang,
Dian Yang
et al.
Abstract:CoFe-based layered double hydroxides (LDHs) are emerging as prominent candidates for the oxygen evolution reaction (OER) due to their tunable 3d orbital electronic structure but are still restricted by the strong adsorption of oxygen-containing intermediates due to their high antibonding orbital relative to the Fermi level. Herein, we synthesized Ga-doped CoFe LDH (GaCoFe LDH) as a highly effective catalyst for alkaline OER. Experimental and theoretical investigations reveal that the strong p−d orbital hybridi… Show more
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