2020
DOI: 10.1021/acs.jpclett.0c02916
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From Reactive Rainbow to Dynamic Resonance Well

Abstract: Scattering resonance is a fascinating phenomenon which manifests as a peak or a dip in an observable as a function of collisional energy (E c). Its occurrence requires a potential well to support the resonance states. In this regard, reactive resonance is unusual in that it can exist in a reaction with unbound Born–Oppenheimer potential energy surface, on which the quasi-bound states are dynamically trappedmeaning that some energy is temporarily tied to the other degrees of freedom than the reaction coordinat… Show more

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Cited by 5 publications
(1 citation statement)
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“…Particle imaging techniques based on Ion Imaging 1 and Velocity Map Imaging (VMI) 2 have revolutionized the field of chemical dynamics, allowing very efficient collection of the velocity distributions of particles coming from a variety of processes. (photodissociation, [1][2][3] photoelectron spectroscopy, 2,4,5 inelastic 6-8 and reactive scattering 9 ) Charged particle-neutral collisions can also be probed [10][11][12] The velocity distributions provide information about the physics underlying and controlling the process of interest. The high collection efficiency is particularly valuable for time-resolved experiments, where many measurements need to be made, and for low count rate experiments.…”
Section: Introductionmentioning
confidence: 99%
“…Particle imaging techniques based on Ion Imaging 1 and Velocity Map Imaging (VMI) 2 have revolutionized the field of chemical dynamics, allowing very efficient collection of the velocity distributions of particles coming from a variety of processes. (photodissociation, [1][2][3] photoelectron spectroscopy, 2,4,5 inelastic 6-8 and reactive scattering 9 ) Charged particle-neutral collisions can also be probed [10][11][12] The velocity distributions provide information about the physics underlying and controlling the process of interest. The high collection efficiency is particularly valuable for time-resolved experiments, where many measurements need to be made, and for low count rate experiments.…”
Section: Introductionmentioning
confidence: 99%