2007
DOI: 10.1140/epjd/e2007-00195-4
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Friction of the surface plasmon by high-energy particle-hole pairs

Abstract: Abstract. We show that the dynamics of the surface plasmon in metallic nanoparticles damped by its interaction with particle-hole excitations can be modelled by a single degree of freedom coupled to an environment. In this approach, the fast decrease of the dipole matrix elements that couple the plasmon to particle-hole pairs with the energy of the excitation allows a separation of the Hilbert space into low-and high-energy subspaces at a characteristic energy that we estimate. A picture of the spectrum consis… Show more

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Cited by 10 publications
(17 citation statements)
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References 29 publications
(93 reference statements)
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“…As can be seen in Fig. 2, the higher the frequency of the mode, the lower is its Landau damping linewidth, similarly to the case of an isolated nanoparticle [35]. Notice also that the dependence of γ σ,L q on the ratio ω 0 /E F is rather weak (thick and thin lines in Fig.…”
Section: A Landau Dampingmentioning
confidence: 53%
“…As can be seen in Fig. 2, the higher the frequency of the mode, the lower is its Landau damping linewidth, similarly to the case of an isolated nanoparticle [35]. Notice also that the dependence of γ σ,L q on the ratio ω 0 /E F is rather weak (thick and thin lines in Fig.…”
Section: A Landau Dampingmentioning
confidence: 53%
“…Whenω 1 /ω 2 = 1, the higher energy + mode is less damped than the lower-energy − one. This energy dependence is analogous to the single nanoparticle case, where higher mode frequencies correspond to lower values of the damping rates [34,35].…”
Section: Nonradiative and Radiative Decay Rates Of The Dark And Bmentioning
confidence: 78%
“…The dipolar LSPs have a dipole moment p = −eN e h(R)p, where e is the electronic charge, N e is the number of valence electrons in each nanoparticle, h(R) is the displacement field associated with the electronic centre-of-mass motion that corresponds to the LSP at position R, and p is the dipole unit vector. The LSP can be regarded as a bosonic mode, in particular when the size of the nanoparticle is small enough such that quantum size effects are important [47][48][49][50][51][52][53][54].…”
Section: Modelmentioning
confidence: 99%