“…Particularly, zero-background Doppler-free scheme, such as polarization spectroscopy [11,12], intermodulated optogalvanic spectroscopy [13,14], intermodulated fluorescence spectroscopy [15], resonance ionization spectroscopy [16] and crossed laser-atomic beam methods [7-10, 17, 18] are powerful techniques to improve spectral SNR for observing weak transitions. One of the method, the two-photon spectroscopy in a power-enhanced cavity, has been successfully achieved for helium 2 1 S 0 − 3 3 D 2 transition [19,20]. Previous investigations of helium energy levels have predominantly been focused on transitions within the triplet manifold, encompassing studies of fine and hyperfine structures, as well as total transition frequencies.…”