2014
DOI: 10.1002/adma.201402682
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Frequency‐Dependent, Alternating Current‐Driven, Field‐Induced Polymer Electroluminescent Devices with High Power Efficiency

Abstract: A significant enhancement in power efficiency for alternating current-driven field-induced polymer electroluminescent devices is demonstrated by employing a high-k ferroelectric polymer dielectric through impedance matching of the device with the driving source. A peak power efficiency of 34.1 lm W(-1) at a frequency of 65 kHz is achieved, which is 2 to 12 times higher than the previous highest reports.

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Cited by 39 publications
(51 citation statements)
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“…The light intensity also increases with alternating-current frequency at a constant voltage bias, and luminance of 2,000 cd m −2 was achieved at 100 kHz. However, very poor light emission was observed at 400 kHz owing to insufficient time for carrier injection, consistent with previous results3132. It should be noted that the device was electrically broken down at the voltage of ∼60 V. The device performance was degraded at 200 kHz, compared with that at 100 kHz and the device failure occurred at ∼60 V, when it was operated both 300 and 400 kHz (Supplementary Fig.…”
Section: Resultssupporting
confidence: 90%
See 1 more Smart Citation
“…The light intensity also increases with alternating-current frequency at a constant voltage bias, and luminance of 2,000 cd m −2 was achieved at 100 kHz. However, very poor light emission was observed at 400 kHz owing to insufficient time for carrier injection, consistent with previous results3132. It should be noted that the device was electrically broken down at the voltage of ∼60 V. The device performance was degraded at 200 kHz, compared with that at 100 kHz and the device failure occurred at ∼60 V, when it was operated both 300 and 400 kHz (Supplementary Fig.…”
Section: Resultssupporting
confidence: 90%
“…To this end, we envisioned that a field-driven organic light-emitting platform would be useful for dynamic interactive display applications. One or two insulating layers can be inserted between the electrode and light-emitting layer, to facilitate carrier injection on alternating-current field2324252627282930313233343536. In addition, this unique architecture with insulating layers does not permit the direct contact between the electrodes and light-emitting layers and thus band alignment design of the two layers may not be necessarily considered.…”
mentioning
confidence: 99%
“…This phenomenon was also observed in purely capacitive electroluminescent devices with organic semiconductor active materials. 64,[71][72][73] The spatial position of the carrier recombination (light emission) zone of the AC-driven PeLEFET can be controlled by modifying the gate or source drain voltages of the device, similarly to its DC-driven counterpart. This can be achieved in both cases of AC-driven drain or gate electrodes.…”
Section: Resultsmentioning
confidence: 99%
“…Existing challenges in the ACEL devices are their high operating voltage and low efficiency, which might impede their applications in wearable and portable electronics. Fortunately, studies are being carried out with promising improvements of reduced operating voltages (< 50 V) and increased efficiency in the organic ACEL devices [46,47]. Different approaches have also been conducted to effectively reduce the operating voltage in the inorganic ACEL devices.…”
Section: Alternating Current Electroluminescence (Acel)mentioning
confidence: 99%