The last few years have highlighted the existence of two relevant length scales in the quest to ultrahigh-strength polycrystalline metals. Whereas the microstructural length scale -e.g. grain or twin size -has mainly be linked to the well-established Hall-Petch relationship, the sample length scale -e.g. nanopillar size -has also proven to be at least as relevant, especially in microscale structures. In this letter, a series of ballistic tests on functionally graded nanocrystalline plates are used as a basis for the justification of a "grain size gradient length scale" as an additional ballistic properties optimization parameter.Recent research works fueled by the recent advances in fabrication processes have emphasized the need to better understand naturally or artificially made size effects in materials in order to enhance their properties [1]. Material strength, more particularly, has been found to be microstructurally linked to two length scales [2], The microstructural length scale -or intrinsic length scale -is related to the size of the material building block micro-or nanostructures. In polycrystalline metals, the most common examples are the grain and/or twin sizes which, refined to the nanometer range (<100«7«), effectively reduce the dislocations mobility, and thus achieve very high yield strength and surface hardness -as predicted by the Hall-Petch equation [3,4]. The second length scale -or extrinsic length scale -is related to the sample size. In metals, the typical example is the ultrahigh strength of monocrystalline nanopillars [5], directly related to the size-dependent scarcity of initial dislocations (starved first before further nucleation [6]).A recent experimental-numerical campaign has highlighted the potential of nanocrystals and nanotwinned ultrafine crystals steel for ballistic protection systems [7]. In this reference, hybridization with a carbon fiber-epoxy composite layer was proposed as a way to improve the nanocrystalline brittleness without dramatically increasing the overall weight. Ultimately, nanocrystalline and nanotwinned ultrafine crystals exhibited a lower ballistic energy absorption than coarse-grained steel, but at equal ballistic limit or weight prior to penetration, deformation in the impact direction was found to be smaller by nearly 40% [7].Surface mechanical attrition treatment (SMAT), the process used for the fabrication of these nanocrystalline and nanotwinned ultrafine crystalline plate, generates a gradient of ultrafine crystal grain sizes ([8,7]). Subsequent coating with a nitriding layer further refines the grains on the top layer to the nanoscale [9,7]. Both processes are nevertheless localized at the surface, leading to a gradient of grain size ranging from the targeted nanocrystals to