Recent organic pollution is caused primarily by the decay of blue-green algae, Microcystis aeruginosa, which is seriously multiplied due to phosphorus-based anthropogenic eutrophication. In eutrophic water, the phenomenon of pH rising in the surface water occurs due to photosynthesis by M. aeruginosa (rising over pH 10). Such pH value is enough to produce calcium phosphate precipitation. The M. aeruginosa cells form colonies and have the outer layer of which is surrounded by a gelatinous sheath. Thus, we considered simultaneous removal of phosphate ion and blue-green algae using calcium chloride from water surface of eutrophic pond. In the present chapter, a simultaneous removal method employing water chemical remediation (WCR) is described. In this method, a flow system was constructed by equipment of a calcium chloride injector and a sand filtration column. As a result, both calcium phosphate and agglutinated algae could be removed from the eutrophic pond water. These water nutrients are removed, phosphorus is concerned about exhaustion as a resource, and the collected algae can be used in various ways as biomass resources. Thus, our system showed the future ability to improve water quality, to remove contaminants, and to recover nutrients from eutrophic water.