First-Principles Calculations Predict Tunable Large Magnetic Anisotropy Due to Spin-Polarized Quantum-Well Resonances in Nanometer-Thick SrRuO₃ Films: Implications for Spintronic Devices

Abstract

We demonstrate that the magnetic anisotropy in SrRuO 3 (SRO) ultrathin films can be well controlled by thickness or electrical modulations: The easy axis (preferred magnetization direction) of a SRO ultrathin film can be switched between out-of-plane and in-plane magnetization either by altering the film thickness or by tuning the doping level through applying a gate voltage or chemical doping. Such a capability to manipulate the magnetocrystalline anisotropy energy (MCAE) is given by the spin−orbit coupling (SOC)induced energy splitting in the spin-polarized quantum well states (QWSs) near the Fermi level. These QWSs are susceptible to the intrinsic spin−orbit interaction and thus drive a large energy discrepancy when an SRO ultrathin film rotates its magnetization direction. As a result of the MCAE nature, a SRO film has a magnetic anisotropy approximately an order of magnitude larger than those in 3d-ferromagnet ultrathin films and its easy-axis direction depends on the film thickness, gate voltage, and substrate. This tunable large magnetic anisotropy in SRO ultrathin films provides an excellent route toward advanced spintronic devices such as storage and memory devices.

Induction of Large Magnetic Anisotropy Energy and Formation of Multiple Dirac States in SrIrO$_3$ Films: Role of correlation and spin-orbit coupling

“…Specific to SIO, we demonstrate the cause of MIT and report the possible existence of multiple Dirac states. Irrespective of layer termination, we show that, these ultrathin films exhibits large MAE which is one to two order higher than the traditional MAE materials like transition metals and their multilayers [26][27][28] .…”

“…It is very rare that oxide films possess large MAE. A very recent theoretical study on SrRuO 3 thin films report a MAE of ≈ 0.62 meV/Ru26 . Also, for comparison, the MAE for other known oxides is summarized in Table-I.…”