“…For designing and application of piezoelectric devices, the materials group of langasite (LGS, La 3 Ga 5 SiO 14 ) with the Ca 3 Ga 2 Ge 4 O 14 (CGG) type crystals structure has merits in terms of piezoelectric properties, which exhibit intermediate values between those of quartz and lithium tantalate [1][2][3]. Compounds such as La 3 Nb 0.5-Ga 5.5 O 14 (LNG) [4], La 3 Ta 0.5 Ga 5.5 O 14 (LTG) [5], Sr 3 NbGa 3 Si 2 O 14 (SNGS) [6,7], Sr 3 TaGa 3 Si 2 O 14 (STGS) [8], Ca 3 NbGa 3 Si 2 O 14 (CNGS) [6,9] and Ca 3 TaGa 3 Si 2 O 14 (CTGS) [10] have been developed for the same purpose based on langasite crystals.…”