“…Thus, harsh reaction conditions, overoxidation, and the deposition of coke could be theoretically avoided. In the past two decades, a wide range of products have been successfully obtained through photocatalytic methane conversion, such as methanol, ethanol, ethane/ethylene, benzene, and syngas, in batch reactors, but with very moderate efficiency due to the following major causes. First, the high recombination rate of photoinduced carriers in the intrinsic semiconductor greatly limits their quantum efficiency, thus resulting in low conversion.…”