We report here on the first direct observations of the vortex lattice in the bulk of electron-doped Nd1.85Ce0.15CuO4 single crystals. Using small angle neutron scattering, we have observed a square vortex lattice with the nearest-neighbors oriented at 45 • from the Cu-O bond direction, which is consistent with theories based on the d-wave superconducting gap. However, the square symmetry persists down to unusually low magnetic fields. Moreover, the diffracted intensity from the vortex lattice is found to decrease rapidly with increasing magnetic field.It is a matter for debate whether hole-doped and electron-doped high-T c cuprate superconductors (HTSC) can be described within a unified physical picture [1,2]. Indeed, electron-doped HTSC have markedly different properties from hole-doped HTSC. For example, electron-doped materials have comparatively low values of the superconducting transition temperature, T c , and much lower values of the upper critical field, B c2 . Furthermore, their normal-state resistivity varies as T 2 as expected for a Fermi-liquid [3,4], and the presence of a pseudogap is still under discussion [5]. Electron-doped HTSC also appear much closer to long-range antiferromagnetic (AF) order, which can in fact coexist with superconductivity [6,7,8,9]. In hole-doped HTSC, the d-wave nature of the order parameter is well-established [10]. However, the evidence for the symmetry of the superconducting gap in electron doped materials (which has important implications for the pairing mechanism [2]) is somewhat contradictory. Earlier measurements of the penetration depth [11] and tunneling experiments [12] supported s-wave symmetry, whereas a d-wave superconducting order parameter is indicated by more recent phase-sensitive [13] and ARPES experiments [14,15]. The electron-doped superconductors are of particular interest in this respect, since they have a tetragonal structure (rather than orthorhombic) and therefore should show pure d-wave behavior, unaffected by admixture of an s-wave component associated with the orthorhombicity [10].Recently, there has been considerable interest in the nature of the vortex lattice (VL) in unconventional superconductors. For instance, vortex cores in d-wave superconductors are predicted to have a distinctive fourfold structure [16,17,18,19,20]. This leads to the expectation that a square VL is formed at high magnetic field, with the nearest-neighbor directions aligned with the nodes of the order parameter. These theoretical predictions are consistent with the small-angle neutron scattering (SANS) observation of a transition from an Abrikosov-like hexagonal VL to a square VL in the hole-doped HTSC YBa 2 Cu 3 O 7 (YBCO) [21]. However, similar measurements on overdoped La 2−x Sr x CuO 4 (LSCO) [22] show a square lattice with nearest neighbors oriented at 45 • to the nodes of the superconducting order parameter. The orientation of the nodal directions in the heavy-fermion superconductor CeCoIn 5 is at present uncertain [23], so it is unclear if the recent SANS observati...