Susumu KuriharaDepartment of Physics, Waseda University, 3-4-1 Okubo, Shinjuku, Tokyo 169-8555, Japan Abstract. We investigate the excitation spectrum and spin conductivity in square lattice antiferromagnets by nonlinear spin-wave theory. We have found that the excitation spectrum have a rotonlike minimum at about 3/4 of the saturation field. The "roton" appears and softens rapidly to zero as a function of the magnetic field as a result of the especially strong three-magnon interactions. For the spin conductivity, it becomes clear that a two-magnon sideband appears for sufficiently strong three-magnon interactions.
IntroductionIn zero magnetic field, square lattice Heisenberg antiferromagnets (SLHAFs) have the Néel structure and three-magnon interactions [1-4] are prohibited. Accordingly, an excitation spectrum at zero field is in good agreements with linear spin-wave (LSW) results with small renormalization [5].In finite magnetic fields, SLHAFs have noncollinear canted states and three-magnon interactions are known to come into play [1][2][3][4]. Moreover, three-magnon interactions can be tuned from zero to quite large values by the external magnetic field. Contrary to the collinear Néel structure, sizable deviations from LSW calculations are pointed out for SLHAFs in high fields both numerically [6,7] and experimentally [8]. Moreover, nonlinear spin-wave spectra are shown to become negative at some wavevectors in high fields [3].Motivated by Ref.[3], we investigate the nonlinear spin-wave spectra within the second-order perturbation calculations based on the formalism of Zhitomirsky-Nikuni-Chernyshev [1, 2, 4]. We focus on the field region just below where we get the negative magnon spectra, near 3/4 of the saturation field, and we find a rotonlike minimum on the acoustic mode which softens rapidly to zero with small increase of fields [9]. We believe that the complete softening of the roton has crucial importance, and a new ground state should appear in higher magnetic fields.We also study the spin conductivity in SLHAFs in fields by the linear response theory since it is expected that the appearance of a "roton" should change thermal and transport properties rather drastically. We compare the results of the LSW calculations [10] and the one with 1/S corrections. A two-magnon sideband appears with 1/S corrections in high fields as a result of the strong three-magnon interactions. We have checked that f-sum rule [10] is satisfied even after the emergence of the sideband.