“…Though the exact mechanism of this observed field-free SOT switching is unclear at present, the Dzyaloshinskii-Moriya interaction (DMI) should play an important role, because both the large difference in interfacial DMI of bottom and top magnetic layers and the additional interlayer DMI can lead to field-free SOT switching in SAFs. [38,39] An in-depth investigation is highly desired and the performance of field-free SOT switching can be further improved via some common approaches, such as exchange bias, interlayer exchange coupling, and tilted sputtering. [36,40,41] Finally, the SOT switching behavior of Type IV (Figure S4b, Supporting Information) is very similar to that of Type I.…”