2020
DOI: 10.1039/d0en00801j
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Few-layered tungsten selenide as a co-catalyst for visible-light-driven photocatalytic production of hydrogen peroxide for bacterial inactivation

Abstract: Sustainable and "green" technologies for hydrogen peroxide (H2O2) production have aroused increasing interests, yet challenges prevail in production of H2O2 for environmental applications. In this study, tungsten selenide (WSe2) with...

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Cited by 34 publications
(25 citation statements)
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“…Hydrogen peroxide (H 2 O 2 ), as a green and highly efficient oxidant used in advanced oxidation processes (AOPs), is commonly produced by an anthraquinone method, an electrochemical method, and photocatalysis. Electro-Fenton (EF) is a new type of AOP, which can generate H 2 O 2 in situ on the surface of the cathode through a two-electron oxygen reduction reaction (ORR) (eq ), avoiding the risk of reagents in transportation, storage, or treatment. , The basic principle of this process is that Fe 2+ added to the solution reacts with the continuously produced H 2 O 2 to form a strong oxidant of hydroxyl radical ( • OH) (eq ); thus, it is efficient and environmentally friendly. However, traditional homogeneous EF has disadvantages such as a narrow pH application range (2.8–3.5), a slow rate of reduction of iron ions, and difficult recovery of the catalyst, which greatly limit its wide application …”
Section: Introductionmentioning
confidence: 99%
“…Hydrogen peroxide (H 2 O 2 ), as a green and highly efficient oxidant used in advanced oxidation processes (AOPs), is commonly produced by an anthraquinone method, an electrochemical method, and photocatalysis. Electro-Fenton (EF) is a new type of AOP, which can generate H 2 O 2 in situ on the surface of the cathode through a two-electron oxygen reduction reaction (ORR) (eq ), avoiding the risk of reagents in transportation, storage, or treatment. , The basic principle of this process is that Fe 2+ added to the solution reacts with the continuously produced H 2 O 2 to form a strong oxidant of hydroxyl radical ( • OH) (eq ); thus, it is efficient and environmentally friendly. However, traditional homogeneous EF has disadvantages such as a narrow pH application range (2.8–3.5), a slow rate of reduction of iron ions, and difficult recovery of the catalyst, which greatly limit its wide application …”
Section: Introductionmentioning
confidence: 99%
“…No any lattice fringe is observed in the SiO 2 region (inset in Figure 1C), indicating that the SiO 2 layer is dominated by the amorphous phase 39,40 . CTAB induces a positively charged surface of Fe 3 O 4 @SiO 2 , and then the RF copolymer as the shell layer is formed over Fe 3 O 4 @SiO 2 via a Stöber-like method 22,39 . The thickness of this shell layer is about 100 nm (Figure 1D).…”
Section: Characterizations Of Mrf Microspheresmentioning
confidence: 99%
“…551) and (440) planes of cubic Fe 3 O 4 , respectively. A broad diffraction band at about 20 o can be attributed to the (002) planes of graphitic carbon, suggesting the presence of πstacking benzenoid-quinoid couples 22,43 . The surface functional groups of MRF were also analyzed by FTIR spectra (Figure 1F).…”
Section: Characterizations Of Mrf Microspheresmentioning
confidence: 99%
“…It is used in photovoltaic devices and ultra-thin LEDs and is an additive in lubricants due to its flake structure with small friction coefficient [11]. The reconfiguration or doping on WSe 2 with other atoms [12] enhances its applications in environmental engineering [13] and chemical engineering [14]. The wide application of nano-WSe 2 increases the possibility of its release into the environment.…”
Section: Introductionmentioning
confidence: 99%