Fe2(MoO4)3 assembled by cross-stacking of porous nanosheets enables a high-performance aluminum-ion battery

Liang, Huanyu; Liu, Yongshuai; Zuo, Fengkai; Zhang, Cunliang; Yang, Li; Zhao, Linyi; Li, Yuhao; Xu, Yifei; Wang, Tiansheng; Hua, Xian-Sheng; Zhu, Yue; Li, Hongsen

doi:10.1039/d2sc05479e

Chem. Sci.

2022

DOI: 10.1039/d2sc05479e

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Fe₂(MoO₄)₃ assembled by cross-stacking of porous nanosheets enables a high-performance aluminum-ion battery

Huanyu Liang

Yongshuai Liu

Fengkai Zuo

et al.

Abstract: Rechargeable aluminum-ion batteries have attracted increasing attention owing to the advantageous multivalent ion storage mechanism thus high theoretical capacity as well as inherent safety and low cost of using aluminum....

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Cited by 8 publications

(1 citation statement)

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“…Liang et al reported a metal oxide, Fe 2 (MoO 4 ) 3 , with excellent stability which was assembled by cross-stacking porous nanosheets. 9 Liu et al proposed and demonstrated the Al-storage mechanism of an alloying reaction with a bimetallic activation center. 10 Li et al tuned the gradients of heteroatoms, N and P, doped in the MOF-derived porous carbon in a C@N–C@N,P–C heterostructure.…”

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SnS₂ quantum dots-coated VO₂@carbon nanorods for secondary battery displaying high capacity and rate-performance

Han,

Wang,

Tao

et al. 2024

Chem. Commun.

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confidence: 99%

SnS₂ quantum dots-coated VO₂@carbon nanorods for secondary battery displaying high capacity and rate-performance

Han,

Wang,

Tao

et al. 2024

Chem. Commun.

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Revealing the Nature of Binary‐Phase on Structural Stability of Sodium Layered Oxide Cathodes

Liu,

Huang,

Liu

et al. 2024

Advanced Materials

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The emergence of layered sodium transition metal oxides featuring a multiphase structure presents a promising approach for cathode materials in sodium‐ion batteries (SIBs), showcasing notably improved energy storage capacity. However, the advancement of cathodes with multiphase structures faces obstacles due to the limited understanding of the integrated structural effects. Herein, we comprehend the integrated structural effects by an in‐depth structure‐chemistry analysis in the developed layered cathode system NaxCu0.1Co0.1Ni0.25Mn0.4Ti0.15O2 with purposely designed P2/O3 phase integration. Our results affirmed that integrated phase ratio plays a pivotal role in electrochemical/structural stability, particularly at high voltage and with the incorporation of anionic redox. In contrast to previous reports advocating solely for the enhanced electrochemical performance in biphasic structures, we demonstrated an inappropriate composite structure is more destructive than a single‐phase design. The in situ X‐ray diffraction (XRD) results, coupled with density functional theory (DFT) computations further confirm the biphasic structure with P2:O3 = 4:6 shows suppressed irreversible phase transition at high desodiated states and thus exhibits optimized electrochemical performance. These fundamental discoveries provide clues to the design of high‐performance layered oxide cathodes for next‐generation SIBs.This article is protected by copyright. All rights reserved

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Preparation of novel authentication film by screen printing of anthocyanin biomolecular extract: Thermochromism and vapochromism

et al. 2023

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Novel thermochromic and vapochromic paper substrates were prepared via screen printing with anthocyanin extract in the presence of ferrous sulfate mordant, resulting in multi‐stimuli responsive colorimetric paper sheets. Environmentally friendly anthocyanin extract was obtained from red‐cabbage (Brassica oleracea var. capitata L.) to function as spectroscopic probe in coordination with ferrous sulfate mordant. Pink anthocyanin/resin nanocomposite films immobilized onto paper surface were developed by well‐dispersion of anthocyanin extract as a colorimetric probe in a binding agent without agglomeration. As demonstrated by CIE colorimetric studies, the pink (λmax = 418 nm) film deposited onto paper surface turns greenish‐yellow (λmax = 552 nm) upon heating from 25 to 75°C, demonstrating new thermochromic film for anti‐counterfeiting applications. The thermochromic effects were investigated at different concentrations of the anthocyanin extract. Upon exposure to ammonia gas, the color of the anthocyanin‐printed sheets changes rapidly from pink to greenish‐yellow, and then immediately returns to pink after taking the gaseous ammonia stimulus away, demonstrating vapochromic effect. The current sensor strip showed a detection limit for ammonia gas in the range 50–300 ppm. Both thermochromism and vapochromism showed high reversibility without fatigue. In addition to studying the rheological properties of the prepared composites, the morphological and mechanical properties of the printed cellulose substrates were also studied.

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Fe₂(MoO₄)₃ assembled by cross-stacking of porous nanosheets enables a high-performance aluminum-ion battery

Abstract: Rechargeable aluminum-ion batteries have attracted increasing attention owing to the advantageous multivalent ion storage mechanism thus high theoretical capacity as well as inherent safety and low cost of using aluminum....

Cited by 8 publications

References 77 publications

SnS₂ quantum dots-coated VO₂@carbon nanorods for secondary battery displaying high capacity and rate-performance

SnS₂ quantum dots-coated VO₂@carbon nanorods for secondary battery displaying high capacity and rate-performance

Revealing the Nature of Binary‐Phase on Structural Stability of Sodium Layered Oxide Cathodes

Preparation of novel authentication film by screen printing of anthocyanin biomolecular extract: Thermochromism and vapochromism

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Fe2(MoO4)3 assembled by cross-stacking of porous nanosheets enables a high-performance aluminum-ion battery

Abstract: Rechargeable aluminum-ion batteries have attracted increasing attention owing to the advantageous multivalent ion storage mechanism thus high theoretical capacity as well as inherent safety and low cost of using aluminum....

Cited by 8 publications

References 77 publications

SnS2 quantum dots-coated VO2@carbon nanorods for secondary battery displaying high capacity and rate-performance

SnS2 quantum dots-coated VO2@carbon nanorods for secondary battery displaying high capacity and rate-performance

Revealing the Nature of Binary‐Phase on Structural Stability of Sodium Layered Oxide Cathodes

Preparation of novel authentication film by screen printing of anthocyanin biomolecular extract: Thermochromism and vapochromism

Contact Info

Product

Resources

About

Fe₂(MoO₄)₃ assembled by cross-stacking of porous nanosheets enables a high-performance aluminum-ion battery

SnS₂ quantum dots-coated VO₂@carbon nanorods for secondary battery displaying high capacity and rate-performance

SnS₂ quantum dots-coated VO₂@carbon nanorods for secondary battery displaying high capacity and rate-performance