Biological materials such as conch shells with crossed-lamellar
textures hold impressive mechanical properties due to their capability
to realize effective crack control and energy dissipation through
the structural synergy of interfacial modulus mismatch and lamellar
orientation disparity. Integrating this mechanism with mechanical
metamaterial design can not only avoid the catastrophic post-yield
stress drop found in traditional architectural materials with uniform
lattice structures but also effectively maintain the stress level
and improve the energy absorption ability. Herein, a novel bioinspired
design strategy that combines regional particularity and overall cyclicity
is proposed to innovate the connotation of long-range periodicity
inside the metamaterial, in which the node constraint gradient and
crossed-lamellar struts corresponding to the core features of conch
shells are able to guide the deformation sequence with a self-strengthening
response during compression. Detailed in situ experiments
and finite element analysis confirm that the rotated broad layer stacking
can shorten and impede the shear bands, further transforming the deformation
of bioinspired metamaterial into a progressive, hierarchical way,
highlighted by the cross-layer hysteresis. Even based on a brittle
polymeric resin, excellent specific energy absorption capacity [4544
kJ/kg] has been achieved in this architecture, which far exceeds the
reported metal-based syntactic foams for two orders of magnitude.
These results offer new opportunities for the bioinspired metamaterials
to substitute the widespread syntactic foams in specific applications
required for both lightweight and energy absorption.