Abstract:Noble metal medium entropy alloy (MEA) thin films have recently attracted enormous research interests recently because of their great potential in the catalytic application. However, conventional bottom‐up fabrication methods for MEA thin film such as magnetron sputtering face enormous challenges including precise control over film thickness and consumption of costly high‐purity noble metal targets. Herein, a facile and tunable approach is developed coupling sequential atomic layer deposition (ALD) of noble me… Show more
“…The feasibility of this method was veried in our previous works. 50,51 The sub-surface area of HEA exhibited partial amorphization and nanocrystallites, which was caused by the explosive crystallization that occurred during the cooling phase of the EJH process. 52,53 The ultrafast ramping/cooling rate also enabled the alloying of multiple layers without encountering phase separation and precipitation.…”
Noble metal-based high entropy alloy (NM-HEA) nanofilm with surface amorphization, synthesized by ALD-EJH method, demonstrates outstanding hydrogen evolution reaction (HER) performance. The experimental and calculational results reveal the mechanism.
“…The feasibility of this method was veried in our previous works. 50,51 The sub-surface area of HEA exhibited partial amorphization and nanocrystallites, which was caused by the explosive crystallization that occurred during the cooling phase of the EJH process. 52,53 The ultrafast ramping/cooling rate also enabled the alloying of multiple layers without encountering phase separation and precipitation.…”
Noble metal-based high entropy alloy (NM-HEA) nanofilm with surface amorphization, synthesized by ALD-EJH method, demonstrates outstanding hydrogen evolution reaction (HER) performance. The experimental and calculational results reveal the mechanism.
A facile, rapid Joule heating protocol for forming amorphous-structured transition metal phosphate electrocatalysts with low overpotentials, fast kinetics, and long-term stability for oxygen evolution reaction (OER).
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