components. [1] They consist of an organic semiconductor thin film patterned between two electrodes, the source and the drain. The semiconductor thin film is in contact with an electrolyte in which a gate electrode is immersed. With application of a gate voltage (V G ), ions from the electrolyte enter the semiconductor, changing its doping state and conductivity, which in turn changes the current that flows between the source and the drain (drain current, I D ). [2] This volumetric doping mechanism is highly efficient, leading to large changes in I D for small changes in V G . As a result, OECTs show very high transconductance (g m = ∂I D /∂V G ), which is a parameter that governs signal amplification. [3] The response time, however, for OECTs is typically quite slow, as ions must penetrate through the entire film. [4] This combination of characteristics makes OECTs suitable for applications in bioelectronics and some areas of large-area electronics, most notably printable electronics. [1,5,6] Recently, the characteristics of OECTs have also led to them being explored as neuromorphic devices. [7,8] These are devices that emulate processing functions observed in biological neural networks and are being developed for computing systems that consume less power and overcome the von Neumann performance bottleneck. [9] An identifying characteristic of biological neural networks is that storage and processing of information is co-located on the same unit. [10] One manifestation of this is Hebbian learning, according to which synaptic connections become more efficient upon repeated stimulation of the postsynaptic by the pre-synaptic neuron (neurons that fire together wire together). [11] This property can be captured in OECTs, when repeated voltage pulses at the gate (the equivalent of the pre-synaptic input) lead to ion accumulation in the semiconductor, thereby have a cumulative effect on the drain current (the post-synaptic output). Leve raging this property, processing functions including synaptic plasticity, orientational selectivity, and homeoplasticity have been demonstrated with OECTs. [7,12,13] Photolithography is still by far the most commonly reported approach for fabricating OECTs. [3,[14][15][16][17] However, the simple structure of OECTs and the ease of formulation of organic materials into different material formats have enabled fabrication using a variety of manufacturing techniques, such as screen printing, spin coating, inkjet printing, and gel extrusion. [18][19][20][21][22] Photolithography is highly efficient, with excellent yields, high achievable resolution, and scalability, but in research and also low-volume, late-stage manufacturing, there is often a greater Organic electrochemical transistors (OECTs) are proving essential in bioelectronics and printed electronics applications, with their simple structure, ease of tunability, biocompatibility, and suitability for different routes to fabrication. OECTs are also being explored as neuromorphic devices, where they emulate characteristics of biologica...