Fabricating penta-coordinated Fe single atoms for electrochemical CO<sub>2</sub>reduction to syngas

Wang, Linjie; Lai, Xiaojing; Xu, Yishen; Luo, Shaojuan; Wang, Lu; Yan, Kai; Zhang, Da; Feng, Sitong; Xu, Yong

doi:10.1039/d3cy00621b

Catal. Sci. Technol.

2023

DOI: 10.1039/d3cy00621b

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Fabricating penta-coordinated Fe single atoms for electrochemical CO₂reduction to syngas

Linjie Wang

Xiaojing Lai

Yishen Xu

et al.

Abstract: The electrochemical reduction of CO2 (CO2RR) has recently attract ed increasing attention for converting intermittent electric energy to chemical energy and reducing CO2 emission. Generally, various products including C1 and...

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Atomically Dispersed Metal Catalysts for the Conversion of CO₂ into High‐Value C₂₊ Chemicals

Yang,

Liu,

Lin

et al. 2024

Advanced Materials

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The conversion of carbon dioxide (CO2) into value‐added chemicals with two or more carbons (C2+) is a promising strategy that can not only mitigate the anthropogenic CO2 emissions but also reduce the excessive dependence on fossil feedstocks. In recent years, atomically dispersed metal catalysts (ADCs), including single‐atom catalysts (SACs), dual‐atom catalysts (DACs) and single‐cluster catalysts (SCCs), emerged as the attractive candidates for CO2 fixation reactions due to their unique properties, such as the maximum utilization of active sites, tunable electronic structure, and the efficient elucidation of catalytic mechanism, etc. In this review, we provide an overview of significant progress in the synthesis and characterization of ADCs utilized in photocatalytic, electrocatalytic and thermocatalytic conversion of CO2 towards high‐value C2+ compounds. To provide insights for designing efficient ADCs towards the C2+ chemical synthesis originating from CO2, the key factors that influence the catalytic activity and selectivity are highlighted. Finally, the relevant challenges and opportunities are discussed to inspire new ideas for the generation of CO2‐based C2+ products over ADCs.This article is protected by copyright. All rights reserved

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Atomically Dispersed Metal Catalysts for the Conversion of CO₂ into High‐Value C₂₊ Chemicals

Yang,

Liu,

Lin

et al. 2024

Advanced Materials

View full text Add to dashboard Cite

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Recent progress of M-N-C single atom electrocatalysts for carbon dioxide reduction reaction

Fauzi,

Chen,

Zhao

et al. 2023

Next Energy

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Recent progress in nickel single-atom catalysts for the electroreduction of CO₂ to CO

Yang,

Chen,

Zhang

et al. 2024

Ind. Chem. Mater.

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Fabricating penta-coordinated Fe single atoms for electrochemical CO₂reduction to syngas

Abstract: The electrochemical reduction of CO2 (CO2RR) has recently attract ed increasing attention for converting intermittent electric energy to chemical energy and reducing CO2 emission. Generally, various products including C1 and...

Cited by 3 publications

References 31 publications

Atomically Dispersed Metal Catalysts for the Conversion of CO₂ into High‐Value C₂₊ Chemicals

Atomically Dispersed Metal Catalysts for the Conversion of CO₂ into High‐Value C₂₊ Chemicals

Recent progress of M-N-C single atom electrocatalysts for carbon dioxide reduction reaction

Recent progress in nickel single-atom catalysts for the electroreduction of CO₂ to CO

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Fabricating penta-coordinated Fe single atoms for electrochemical CO2reduction to syngas

Abstract: The electrochemical reduction of CO2 (CO2RR) has recently attract ed increasing attention for converting intermittent electric energy to chemical energy and reducing CO2 emission. Generally, various products including C1 and...

Cited by 3 publications

References 31 publications

Atomically Dispersed Metal Catalysts for the Conversion of CO2 into High‐Value C2+ Chemicals

Atomically Dispersed Metal Catalysts for the Conversion of CO2 into High‐Value C2+ Chemicals

Recent progress of M-N-C single atom electrocatalysts for carbon dioxide reduction reaction

Recent progress in nickel single-atom catalysts for the electroreduction of CO2 to CO

Contact Info

Product

Resources

About

Fabricating penta-coordinated Fe single atoms for electrochemical CO₂reduction to syngas

Atomically Dispersed Metal Catalysts for the Conversion of CO₂ into High‐Value C₂₊ Chemicals

Atomically Dispersed Metal Catalysts for the Conversion of CO₂ into High‐Value C₂₊ Chemicals

Recent progress in nickel single-atom catalysts for the electroreduction of CO₂ to CO