Abstract:Reducing global carbon dioxide emissions is a critical issue that requires sustainable, energy-efficient and scalable solutions. Electrochemical carbon dioxide capture and release with redox active molecule has drawn an intense amount of interest, owing to its mild operation condition, low energy consumption and high flexibility compared with traditional CO2 capture technologies. Here, we demonstrate a series of thiolate/ disulfide redox couples, with high practical solubility and weak protonation ability, whi… Show more
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