2023
DOI: 10.1039/d3nr03497f
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Exceptional ultrafast nonlinear optical response of functionalized silicon nanosheets

Michalis Stavrou,
Amelie M. Mühlbach,
Vasilios Arapakis
et al.

Abstract: This study reveals that the functionalization of silicon nanosheets with styrene and tBuMA leads to nanostructures with exceptional nonlinear optical response. These nanostructures could have potential applications in optoelectronics and photonics.

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Cited by 3 publications
(2 citation statements)
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References 82 publications
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“…Fitting this peak with a Gaussian-type function provides the autocorrelation profile of the laser, which showed a pulse width of approximately 260 fs. The adjacent, more intense peak corresponds to the contribution of molecular reorientation on the NLO response, which is followed by an exponential-like decay of the molecular system as it relaxes toward the equilibrium. , …”
Section: Resultsmentioning
confidence: 99%
“…Fitting this peak with a Gaussian-type function provides the autocorrelation profile of the laser, which showed a pulse width of approximately 260 fs. The adjacent, more intense peak corresponds to the contribution of molecular reorientation on the NLO response, which is followed by an exponential-like decay of the molecular system as it relaxes toward the equilibrium. , …”
Section: Resultsmentioning
confidence: 99%
“…Researchers have developed various passive optical limiters based on nonlinear mechanisms, including saturable and reverse saturable absorption, two-photon absorption, and multiphoton absorption. 11–15 However, the current issue with existing optical limiters is that their working principle, based on nonlinear optical effects, demands relatively high intensity radiation. 16 Consequently, the transmittance of an optical limiter begins to decrease at a much higher level of incident radiation than is required for optical sensor protection in most cases.…”
Section: Introductionmentioning
confidence: 99%