Abstract:We have been attempting to develop the numerical model for mercury fate in Minamata Bay and Yatsushiro Sea. In this paper we compared numerical results of bottom sediment transport from the bay to the outer sea area for one year with and without sea water and freshwater stratification. As a result, it was clarified that long term bottom sediment transport was determined by both of barotropic currents and baroclinic ones. Thus, accurate numerical model for particulate mercury fate must take into account barocli… Show more
“…Overall, in the horizontal direction, the T-Hg concentration became smaller and smaller along A and B lines from the sampling point Y28, indicating the mercury transport from Minamata Bay to the Yatsushiro Sea. The sediment migration along line A is considered to be mainly affected by barotropic current, while the sediment migration along line B mainly influenced by baroclinic current, consistent with the findings by Yano et al 19) . In the vertical direction, the T-Hg concentration increased first and then decreased overall.…”
Section: (3) the Total Mercury Concentrations Of Different Particle S...supporting
After the outbreak of Minamata Disease, highly mercury-polluted sediment was dredged from Minamata Bay. Nevertheless, some studies indicated that trace mercury (Hg) migrated from Minamata Bay to the Yatsushiro Sea with the movement of sediments. Mercury was considered to adsorb on sediment particles and realized the transport. However, the influence of particle size as a crucial factor affecting adsorption is barely considered in the analysis of mercury migration.In this study, we develop a novel method based on particle size classification to comprehend both horizontal and vertical distribution of the total-Hg (T-Hg) concentration in sediments with different particle sizes in the Yatsushiro Sea. From the experiment result, it could be concluded that overall, in the horizontal direction, the T-Hg concentration became smaller and smaller along A and B lines from the sampling point Y28, indicating the mercury transport from Minamata Bay to the Yatsushiro Sea. Moreover, the T-Hg concentration increased first and then decreased in the vertical direction, suggesting that the migrated mercury was mainly deposited in the upper sediments. Furthermore, according to the classification experiment results, the smaller the particle size, the higher the T-Hg concentration. And, the sediment particles migrating from Minamata Bay to the Yatsushiro Sea are mainly very fine slit to fine silt.
“…Overall, in the horizontal direction, the T-Hg concentration became smaller and smaller along A and B lines from the sampling point Y28, indicating the mercury transport from Minamata Bay to the Yatsushiro Sea. The sediment migration along line A is considered to be mainly affected by barotropic current, while the sediment migration along line B mainly influenced by baroclinic current, consistent with the findings by Yano et al 19) . In the vertical direction, the T-Hg concentration increased first and then decreased overall.…”
Section: (3) the Total Mercury Concentrations Of Different Particle S...supporting
After the outbreak of Minamata Disease, highly mercury-polluted sediment was dredged from Minamata Bay. Nevertheless, some studies indicated that trace mercury (Hg) migrated from Minamata Bay to the Yatsushiro Sea with the movement of sediments. Mercury was considered to adsorb on sediment particles and realized the transport. However, the influence of particle size as a crucial factor affecting adsorption is barely considered in the analysis of mercury migration.In this study, we develop a novel method based on particle size classification to comprehend both horizontal and vertical distribution of the total-Hg (T-Hg) concentration in sediments with different particle sizes in the Yatsushiro Sea. From the experiment result, it could be concluded that overall, in the horizontal direction, the T-Hg concentration became smaller and smaller along A and B lines from the sampling point Y28, indicating the mercury transport from Minamata Bay to the Yatsushiro Sea. Moreover, the T-Hg concentration increased first and then decreased in the vertical direction, suggesting that the migrated mercury was mainly deposited in the upper sediments. Furthermore, according to the classification experiment results, the smaller the particle size, the higher the T-Hg concentration. And, the sediment particles migrating from Minamata Bay to the Yatsushiro Sea are mainly very fine slit to fine silt.
“…Meanwhile, mercury exceeding 0.5 ppm is distributed within about 100 km 2 southwest direction from Minamata Bay, while it is only distributed within about 55 km 2 northeast direction from Minamata Bay. Southwest direction from Minamata Bay is considered to be mainly affected by barotropic current, while northeast direction by baroclinic current 17) . Meanwhile, the bottom slope in the southwest direction from Minamata Bay is generally smaller than that in the northeast direction (Fig.…”
Section: (3) Migration Of Mercury-containing Sediments With Different...mentioning
After Minamata disease occurred in Kumamoto Prefecture, the Minamata Bay Pollution Prevention Project on Minamata Bay area was started to deal with mercury pollution. Beneficial from the project, the mercury content in the bay area has been significantly reduced. However, many studies have shown that the residual trace mercury content around the bay is still high. Furthermore, mercury has migrated from Minamata Bay to the Yatsushiro Sea. Therefore, continuous research on the distribution and content of mercury in this region is required.In this study, using sediment classification, the relationship between sediment particle size, particle specific surface area, and T-Hg (total mercury) concentration was investigated. Based on the numerical simulation, the particle size effect on the migration of mercury-containing sediments and the T-Hg distribution in the Yatsushiro Sea were studied. The result showed that the larger the particle size, the lower the T-Hg concentration in the sediment. Meanwhile, the larger the particle specific surface area, the higher the T-Hg concentration. Moreover, the smaller the particle size of the mercury-containing sediment, the higher the migration speed as well as the more comprehensive migration range. From the numerical simulation results, it was found that mercury was mainly distributed in the southwest and northeast directions from Minamata Bay. Finally, the simulated mercury distribution, which considers the relationship between particle size and mercury concentration, shows a high agreement with the past measurements of mercury, suggesting the importance of particle size effect in mercury migration.
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