2007
DOI: 10.1103/physrevb.75.195404
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Evidence for pore surface dependent positronium thermalization in mesoporous silica/hybrid silica films

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Cited by 50 publications
(30 citation statements)
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“…However, it is true that the cooling rate decreases as cooling proceeds, so that at some point an additional cooling mechanism may be required. This could be laser cooling, or it could be modified collisional cooling, which can be achieved by introducing low mass molecules that increase the energy loss per collision [280]. Other avenues may also be possible: for example, the availability of narrow velocity distributions hinted at by MOF measurements [124] is a promising area for future research, especially considering the huge number of possible MOF materials.…”
Section: Discussionmentioning
confidence: 99%
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“…However, it is true that the cooling rate decreases as cooling proceeds, so that at some point an additional cooling mechanism may be required. This could be laser cooling, or it could be modified collisional cooling, which can be achieved by introducing low mass molecules that increase the energy loss per collision [280]. Other avenues may also be possible: for example, the availability of narrow velocity distributions hinted at by MOF measurements [124] is a promising area for future research, especially considering the huge number of possible MOF materials.…”
Section: Discussionmentioning
confidence: 99%
“…This work has also led to the use of thin mesoporous films that can be used as Ps converters [109,110,[246][247][248][279][280][281][282][283][284]. These materials produce Ps in a similar way to the powders discussed previously [35,36].…”
Section: Ps Productionmentioning
confidence: 99%
“…The lifetime of a fraction of o-Ps is shortened in the nanoporosities by pick-off annihilation, in which the positron of the o-Ps annihilates with an electron of the walls of the pores into 2 c-rays. Porous silica has proved to be a good choice for converting positrons into cold positronium due to the large Ps yield in the bulk and on the porous surface, combined with the relatively efficient cooling of o-Ps by collisions with the walls of the pores [17][18][19].…”
Section: Introductionmentioning
confidence: 99%
“…Length L and diameter d of the pore (framed as a cylinder) can be correlated to the number k of collisions: a stochastic approximation for the random walk of a Ps colliding against the walls of the pore and diffusing toward the open end supplies the relation L = d √ k. Within the same approximation the travel time t is related to the pore diameter d and to the average Ps speed v: t = kd √ 2/v. Travel time and average Ps speed can be assumed t ≈ τ oPs /10, v = 4 × 10of collisions strongly depends on the effective mass of atoms on pore walls: we can estimate for k a range k = 1 × 10 5 −3 × 10 5 [16]. With the above data we obtain d ≈ 4-12 nm and L ≈ 2−4 µm.…”
Section: Positron To Ps Conversionmentioning
confidence: 71%