Entropy-Driven Hybrid Gel Electrolyte Enables Practical High-Voltage Lithium Metal Batteries
Chuyang Jing,
Ziyu Peng,
Kunyun Yan
et al.
Abstract:Electrolyte engineering plays a crucial role in enhancing the performance of lithium metal batteries (LMBs) featuring high-voltage cathodes and limited lithium anodes, thereby unlocking their potential for high-energy electrochemical storage. Herein, an entropy-driven hybrid gel electrolyte with enhanced diversity in Li-ion solvation structures is designed by incorporating substantial amounts of insoluble LiPO 2 F 2 and LiNO 3 salts into LiPF 6 -based carbonate electrolytes, followed by in situ thermal polymer… Show more
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