A model for the concentration of the solute in the gas in a packed column with a countercurrent flow of gas and liquid was developed. The mass-transfer coefficient was needed for the model solution. A 0.61 m diameter column filled with 38-mm ceramic Intalox saddles was used to measure mass-transfer coefficients of air-water and air-carboxymethylcellulose (CMC) solution systems. A 1.2 m diameter column filled with 50-mm ceramic Intalox saddles was also used with an air and calcium chloride solution. For varied flow rates of air from 1422 to 8017 kg m -2 h -1 and water (or the CMC solution) from 3888 to 15 516 kg m -2 h -1 , the measured concentrations of water vapor in air at the bed exit were within 2% with the model prediction. For the aircalcium chloride solution with air flow rates of 1872-7740 kg m -2 h -1 and liquid rates of 12 276-45 980 kg m -2 h -1 , the average deviation between the measured concentrations and the predicted values was about 9%.