We reconstruct Frédéric Joliot and Irène Curie's discovery of artificial radioactivity in January 1934 based in part on documents preserved in the Joliot-Curie Archives in Paris, France. We argue that their discovery followed from the convergence of two parallel lines of research, on the neutron and on the positron, that were focused on a well-defined experimental problem, the nuclear transmutation of aluminum and other light elements. We suggest that a key role was played by a suggestion that Francis Perrin made at the seventh Solvay Conference at the end of October 1933, that the alpha-particle bombardment of aluminum produces an intermediate unstable isotope of phosphorus, which then decays by positron emission. We also suggest that a further idea that Perrin published in December 1933, and the pioneering theory of beta decay that Enrico Fermi also first published in December 1933, established a new theoretical framework that stimulated Joliot to resume the researches that he and Curie had interrupted after the Solvay Conference, now for the first time using a GeigerMüller counter to detect the positrons emitted when he bombarded aluminum with polonium alpha particles. Matteo Leone is contract researcher in the Department of Physics of the University of Genoa; his main fields of research are the history of spectroscopy, atomic physics, nuclear physics, and scientific instruments. Nadia Robotti is Professor of History of Physics in the Department of Physics of the University of Genoa; her main fields of research are the history of atomic physics, quantum mechanics, nuclear physics, and scientific instruments. 3 du Radium; Geiger-Müller counter; beta decay; artificial radioactivity; history of nuclear physics.
IntroductionJean Perrin communicated Irène Curie and Frédéric Joliot's report on their discovery of artificial radioactivity to the Paris Academie des Sciences on January 15, 1934, 1 which gained worldwide attention when it was reported in the February 10 issue of Nature. 2 Science News emphasized that, "Never before [had] radioactivity been created by an external cause," 3 and Ernest Rutherford declared:[It] is remarkable that the life of the unstable atom produced is as long as it is. We do not know whether the atoms so far made artificially radioactive are typical or whether other unstable atoms which may be produced will have a longer or shorter life. The discovery of the Joliots shows how little we really know about radioactivity. 4That became clear in March 1934 when Enrico Fermi in Rome demonstrated that artificial radioactivity was also produced when neutrons bombard elements of high atomic number. 5While Joliot and Curie's discovery of artificial radioactivity has been discussed earlier by historians and physicists, most do not go into detail regarding its timing, 6 or do not offer an explanation for its timing. 7 Joliot first observed artificial radioactivity on the afternoon of January 11, 1934, 8 but in retrospect it seems that it could have been discovered soon after the seventh Solvay Conf...