Enhancing biomass oxidation with carbon nitride nanosheets ring inserted on C. I. Pigment Yellow 53 photocatalysts for simultaneous CO and lactic acid production

Ling, Weikang; Ma, Jiliang; Liu, Zhendong; Cui, Rui; Zhang, Junqiang; Li, Xinze; Hong, Min; Sun, Runcang

doi:10.1016/j.cej.2023.146117

Chemical Engineering Journal

2023

DOI: 10.1016/j.cej.2023.146117

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Enhancing biomass oxidation with carbon nitride nanosheets ring inserted on C. I. Pigment Yellow 53 photocatalysts for simultaneous CO and lactic acid production

Weikang Ling,

Jiliang Ma,

Zhendong Liu

et al.

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2024

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Cited by 7 publications

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Enhancing Photocatalytic Activity for Solar‐to‐Fuel Conversion: A Study on S‐Scheme AgInS₂/CeVO₄@Biochar_x Heterojunctions

Zhang,

Ling,

et al. 2024

Adv Funct Materials

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Rare earth vanadates are promising for solar‐to‐fuel conversions, yet their photocatalytic efficiency is limited by the substantial recombination of photo‐generated carriers. Constructing heterojunctions is recognized as an effective approach to improving charge carrier separation in vanadates. Nonetheless, inefficient charge transfer often results from the poor quality of interfaces and non‐directional charge transfer within these heterojunctions. Herein, an S‐scheme AgInS2/CeVO4@Biocharx (AIS/CV@Cx) heterojunction photocatalyst is designed and synthesized through a straightforward freeze‐drying and calcination three‐step process, aimed at photocatalytic co‐production of xylonic acid and carbon monoxide (CO) from xylose. The AIS/CV@C2 heterojunction achieves an optimal yield of 67.74% for xylonic acid and a CO release of 29.76 µmol from xylose. The enhanced photocatalytic performance of the AIS/CV@C2 heterojunction is attributed to three key factors: I) the high‐quality interface and intimate contact within the AIS/CV@C2 heterojunction significantly reduce undesirable carriers recombination, II) the staggered band structures and directed carriers transfer in the AIS/CV@C2 heterojunction notably improve spatial carriers separation/migration, and III) the incorporation of biochar boosts the conductivity of the AIS/CV@C2 heterojunction. This work presents a straightforward yet effective method for fabricating vanadate heterojunctions, highlighting the importance of quality interfacial contact and directed charge transfer in amplifying photocatalytic performance.

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Enhancing Photocatalytic Activity for Solar‐to‐Fuel Conversion: A Study on S‐Scheme AgInS₂/CeVO₄@Biochar_x Heterojunctions

Zhang,

Ling,

et al. 2024

Adv Funct Materials

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Plasmonic quantum dots modulated nano-mineral toward photothermal reduction of CO2 coupled with biomass conversion

Cao,

Xing,

Gui

et al. 2024

Nano Res.

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Extended H-bonds/π-bonds networks for boosting electron transfer over polydopamine-covered nanocellulose/g-C3N4 toward efficient photocatalytic H2O2 production

Shan,

Wang,

Luo

et al. 2024

Applied Catalysis B: Environment and Energy

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Enhancing biomass oxidation with carbon nitride nanosheets ring inserted on C. I. Pigment Yellow 53 photocatalysts for simultaneous CO and lactic acid production

Cited by 7 publications

References 45 publications

Enhancing Photocatalytic Activity for Solar‐to‐Fuel Conversion: A Study on S‐Scheme AgInS₂/CeVO₄@Biochar_x Heterojunctions

Enhancing Photocatalytic Activity for Solar‐to‐Fuel Conversion: A Study on S‐Scheme AgInS₂/CeVO₄@Biochar_x Heterojunctions

Plasmonic quantum dots modulated nano-mineral toward photothermal reduction of CO2 coupled with biomass conversion

Extended H-bonds/π-bonds networks for boosting electron transfer over polydopamine-covered nanocellulose/g-C3N4 toward efficient photocatalytic H2O2 production

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Enhancing biomass oxidation with carbon nitride nanosheets ring inserted on C. I. Pigment Yellow 53 photocatalysts for simultaneous CO and lactic acid production

Cited by 7 publications

References 45 publications

Enhancing Photocatalytic Activity for Solar‐to‐Fuel Conversion: A Study on S‐Scheme AgInS2/CeVO4@Biocharx Heterojunctions

Enhancing Photocatalytic Activity for Solar‐to‐Fuel Conversion: A Study on S‐Scheme AgInS2/CeVO4@Biocharx Heterojunctions

Plasmonic quantum dots modulated nano-mineral toward photothermal reduction of CO2 coupled with biomass conversion

Extended H-bonds/π-bonds networks for boosting electron transfer over polydopamine-covered nanocellulose/g-C3N4 toward efficient photocatalytic H2O2 production

Contact Info

Product

Resources

About

Enhancing Photocatalytic Activity for Solar‐to‐Fuel Conversion: A Study on S‐Scheme AgInS₂/CeVO₄@Biochar_x Heterojunctions

Enhancing Photocatalytic Activity for Solar‐to‐Fuel Conversion: A Study on S‐Scheme AgInS₂/CeVO₄@Biochar_x Heterojunctions