Most mono-propellant thruster technologies were developed in the 1960s and the basic principles and fundamental structures, such as the catalyst and propellant, have remained in use without major technical innovation. Conversely, much remains to be identified in terms of the concrete mechanisms and quantitative limitations of the phenomena inside the monopropellant thruster. One of our studies to improve the reliability of propulsion systems involved visualization, facilitating direct observation of the physical and chemical phenomena occurring within the catalyst bed of the mono-propellant thruster. In this paper, we introduce the visualization test results of the mono-propellant thruster utilizing Neutron Radiography. We have also succeeded in shooting movies of hydrazine decomposition phenomena using Neutron Radiography at the Kyoto University Research Reactor.