Emerging Antiferromagnets for Spintronics

Abstract

Antiferromagnets constitute promising contender materials for next‐generation spintronic devices with superior stability, scalability, and dynamics. Nevertheless, the perception of well‐established ferromagnetic spintronics underpinned by spontaneous magnetization seemed to indicate the inadequacy of antiferromagnets for spintronics—their compensated magnetization has been perceived to result in uncontrollable antiferromagnetic order and subtle magnetoelectronic responses. However, remarkable advancements have been achieved in antiferromagnetic spintronics in recent years, with consecutive unanticipated discoveries substantiating the feasibility of antiferromagnet‐centered spintronic devices. It is emphasized that, distinct from ferromagnets, the richness in complex antiferromagnetic crystal structures is the unique and essential virtue of antiferromagnets that can open up their endless possibilities of novel phenomena and functionality for spintronics. In this Perspective, the recent progress in antiferromagnetic spintronics is reviewed, with a particular focus on that based on several kinds of antiferromagnets with special antiferromagnetic crystal structures. The latest developments in efficiently manipulating antiferromagnetic order, exploring novel antiferromagnetic physical responses, and demonstrating prototype antiferromagnetic spintronic devices are discussed. An outlook on future research directions is also provided. It is hoped that this Perspective can serve as guidance for readers who are interested in this field and encourage unprecedented studies on antiferromagnetic spintronic materials, phenomena, and devices.

TaF4: A Novel Two-Dimensional Antiferromagnetic Material with a High Néel Temperature Investigated Using First-Principles Calculations

“…Two-dimensional (2D) antiferromagnetic (AFM) materials, which have traditionally been emphasized less in spintronics compared to two-dimensional ferromagnetic materials, have gained significant attention in recent years due to their atomic arrangement, structural characteristics, and exceptional physical properties [ 1 , 2 , 3 , 4 ]. Their magnetic moments are arranged anti-parallel in a two-dimensional plane, forming an ordered magnetic structure [ 5 ].…”