The treatment of dye-contaminated wastewater using granular
sludge
was evaluated to ensure an effective design process for biogranulation
technology. The investigation of dye-contaminated wastewater treatment
in a sequencing batch reactor (SBR) aimed to understand the decolorization
of mixed azo dyes (MAD) mediated by aerobic granular sludge (AGS)
and magnetic-activated carbon aerobic granular sludge (MACAGS). The
applicability of Generalized Fulazzaky equations was expanded to predict
the mechanisms and kinetics of global, external, and internal mass
transfer. The performance of SBR in decolorizing MAD with AGS and
MACAGS reached 65.04% and 82.32% efficiency, respectively, exhibiting
an increased efficiency of 17.28% (82.32–65.04%) with the presence
of magnetic-activated carbon (MAC) in the formation of AGS. A trend
in the variation of the internal mass transfer factor was similar
to that of the global mass transfer factor and was far higher than
that of the external mass transfer factor, indicating that the rate-limiting
step of MAD decolorization was dependent on the resistance of external
mass transfer. An analysis of the decolorization efficiency based
on the internal mass transfer factor provided new insights into the
role of MAC in enhancing the SBR performance, contributing to the
advanced treatment of dye-contaminated wastewater.