2022
DOI: 10.1088/1367-2630/ac8014
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Electrostatic focusing of cold and heavy molecules for the ACME electron EDM search

Abstract: The current best upper limit for electron electric dipole moment (EDM), |de|<1.1×10-29 e·cm (90% confidence), was set by the ACME collaboration in 2018. The ACME experiment uses a spin-precession measurement in a cold beam of ThO molecules to detect de. An improvement in statistical uncertainty would be possible with more efficient use of molecules from the cryogenic buffer gas beam source. Here, we demonstrate electrostatic focusing of the ThO beam with a hexapole lens. This results in a factor of 16 enhan… Show more

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Cited by 9 publications
(3 citation statements)
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“…The gas was cooled down by 17 K neon buffer gas, forming a cryogenic molecular beam mostly in the ground (X ) electronic state [32]. The molecules in the beam were then excited to the Q state using Stimulated Raman Adiabatic Passage (STIRAP) via X-C-Q transitions [33] and were collimated by an electrostatic molecular lens to the readout region downstream [34]. The molecules in the Q state were resonantly excited to the I state by a 746 nm continuous-wave laser (M Squared SolsTis), which decays quickly (lifetime 115 ± 4 ns [35]) to the ground state X, emitting 512 nm photons.…”
Section: Molecular Fluorescence Measurementmentioning
confidence: 99%
“…The gas was cooled down by 17 K neon buffer gas, forming a cryogenic molecular beam mostly in the ground (X ) electronic state [32]. The molecules in the beam were then excited to the Q state using Stimulated Raman Adiabatic Passage (STIRAP) via X-C-Q transitions [33] and were collimated by an electrostatic molecular lens to the readout region downstream [34]. The molecules in the Q state were resonantly excited to the I state by a 746 nm continuous-wave laser (M Squared SolsTis), which decays quickly (lifetime 115 ± 4 ns [35]) to the ground state X, emitting 512 nm photons.…”
Section: Molecular Fluorescence Measurementmentioning
confidence: 99%
“…The hexapole lens was developed for BaF molecules in the first excited rotational level (N = 1) of the electronic and vibrational ground state and has also been tested with molecules in the second excited rotational state (N = 2) state, that may be used as an upgrade to the experiment in the future. In a related study, Wu et al used a hexapole lens to enhance the molecular flux of ThO molecules for the ACME experiment [15].…”
Section: Introductionmentioning
confidence: 99%
“…Figure 1 shows the apparatus for ACME III. A cryogenic buffer-gas beam source generates a cold ThO beam, and hexapole electrodes focus that beam into the interaction region increasing the number of detected molecules [5]. At the entrance of the spin precession region, molecules are optically driven into the H state for the eEDM measurement, where the unpaired electron spins precess in combined electric and magnetic fields.…”
Section: Introductionmentioning
confidence: 99%