Electronic Doppler effect in resonant Auger decay of CO molecules upon excitation near a shake-up<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>Π</mml:mi></mml:math>resonance

Sörensen, Stacey Ristinmaa; Kitajima, M.; Tanaka, Takahiro; Hoshino, M.; Tanaka, Hiroshi; Tamenori, Y.; Sankari, R.; Piancastelli, Maria Novella; Ueda, Kiyoshi; Velkov, Yasen; Minkov, I. M.; Carravetta, Vincenzo; Gel’mukhanov, Faris

doi:10.1103/physreva.76.062704

Phys. Rev. A

2007

DOI: 10.1103/physreva.76.062704

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Electronic Doppler effect in resonant Auger decay of CO molecules upon excitation near a shake-upΠresonance

Stacey Ristinmaa Sörensen

M. Kitajima

Takahiro Tanaka

et al.

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Cited by 7 publications

(1 citation statement)

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“…This effect has been revealed by using linearly polarized light, first in experiments performed with angular selectivity [17][18][19] or, more recently, with full angular resolution [20]. The experimental Doppler profiles of the fragment lines may serve as a fingerprint of nuclear dynamics [8,14] and are widely used in investigations of ultrafast dissociation processes in core-excited states [8,9,15,[17][18][19][20][21][22][23][24][25].…”

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confidence: 99%

Circularly Polarized X Rays: Another Probe of Ultrafast Molecular Decay Dynamics

et al. 2010

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Dissociative nuclear motion in core-excited molecular states leads to a splitting of the fragment Auger lines: the Auger-Doppler effect. We present here for the first time experimental evidence for an Auger-Doppler effect following F1s → a(1g)* inner-shell excitation by circularly polarized x rays in SF(6). In spite of a uniform distribution of the dissociating S-F bonds near the polarization plane of the light, the intersection between the subpopulation of molecules selected by the core excitation with the cone of dissociation induces a strong anisotropy in the distribution of the S-F bonds that contributes to the scattering profile measured in the polarization plane.

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Circularly Polarized X Rays: Another Probe of Ultrafast Molecular Decay Dynamics

et al. 2010

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Ultrafast dissociation: An unexpected tool for probing molecular dynamics

Morin

Miron

2012

Journal of Electron Spectroscopy and Related Phenomena

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Dissociation of core-valence doubly excited states in NO followed by atomic Auger decay

Hikosaka

Kaneyasu²,

Matsushita

et al. 2010

The Journal of Chemical Physics

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The decay processes of core-valence doubly excited states near the N K edge of NO have been studied using electron spectroscopy. Electron yields measured as a function of photon energy and kinetic energy enable the clear identification of atomic Auger lines associated with the dissociation of doubly excited states. The atomic Auger lines exhibit Doppler profiles, allowing the entire reaction scheme of such dissociation processes to be determined.

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Electronic Doppler effect in resonant Auger decay of CO molecules upon excitation near a shake-upΠresonance

Cited by 7 publications

References 40 publications

Circularly Polarized X Rays: Another Probe of Ultrafast Molecular Decay Dynamics

Circularly Polarized X Rays: Another Probe of Ultrafast Molecular Decay Dynamics

Ultrafast dissociation: An unexpected tool for probing molecular dynamics

Dissociation of core-valence doubly excited states in NO followed by atomic Auger decay

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