“…( 3) we find two parameters: ∆ B = 28 mT and B exch = 5.5 mT. The strength of the hyperfine interaction is in good agreement with measurements of optical spin orientation in transverse and longitudinal magnetic fields in a similar sample [25,30], which supports our interpretation. Using the electron g factor g e = 2 [31,32], we find the splitting between bright and dark states δ 0 = 0.6 µeV.…”
supporting
confidence: 88%
“…Experiment -For experimental demonstration of the suggested mechanism we choose the momentum-indirect (In,Al)As/AlAs QDs. Recently, we showed that in these QDs at low temperatures the exciton spin relaxation is dominated by the hyperfine interaction with ∆ B being a few millitesla [25], while the exciton lifetime reaches hundreds of microseconds [26,27]. The QDs have type-I band alignment (both electron and hole are localized inside the QD) [28,29].…”
We suggest a new spin orientation mechanism for localized electrons: dynamic electron spin polarization provided by nuclear spin fluctuations. The angular momentum for the electrons is gained from the nuclear spin system via the hyperfine interaction in a weak magnetic field. For this the sample is illuminated by an unpolarized light, which directly polarizes neither the electrons nor the nuclei. We predict, that for the electrons bound in localized excitons 100% spin polarization can be reached in longitudinal magnetic fields of a few millitesla. The proof of principle experiment is performed on momentum-indirect excitons in (In,Al)As/AlAs quantum dots, where in a magnetic field of 17 mT the electron spin polarization of 30% is measured.
“…( 3) we find two parameters: ∆ B = 28 mT and B exch = 5.5 mT. The strength of the hyperfine interaction is in good agreement with measurements of optical spin orientation in transverse and longitudinal magnetic fields in a similar sample [25,30], which supports our interpretation. Using the electron g factor g e = 2 [31,32], we find the splitting between bright and dark states δ 0 = 0.6 µeV.…”
supporting
confidence: 88%
“…Experiment -For experimental demonstration of the suggested mechanism we choose the momentum-indirect (In,Al)As/AlAs QDs. Recently, we showed that in these QDs at low temperatures the exciton spin relaxation is dominated by the hyperfine interaction with ∆ B being a few millitesla [25], while the exciton lifetime reaches hundreds of microseconds [26,27]. The QDs have type-I band alignment (both electron and hole are localized inside the QD) [28,29].…”
We suggest a new spin orientation mechanism for localized electrons: dynamic electron spin polarization provided by nuclear spin fluctuations. The angular momentum for the electrons is gained from the nuclear spin system via the hyperfine interaction in a weak magnetic field. For this the sample is illuminated by an unpolarized light, which directly polarizes neither the electrons nor the nuclei. We predict, that for the electrons bound in localized excitons 100% spin polarization can be reached in longitudinal magnetic fields of a few millitesla. The proof of principle experiment is performed on momentum-indirect excitons in (In,Al)As/AlAs quantum dots, where in a magnetic field of 17 mT the electron spin polarization of 30% is measured.
“…For simplicity we neglect a number of contributions in the Hamiltonian. First, we neglect the long range electron hole exchange interaction, which is suppressed for the indirect excitons [31][32][33] as well as possible noncollinear terms in the short range exchange interaction for electrons in the X valley. We also neglect the hole Zeeman splitting, because the transverse components of the tensor of the heavy hole g factors are very small [34,35], while the longitudinal component does not play a role in the phenomena addressed here [11].…”
Section: A Modelmentioning
confidence: 99%
“…For simplicity we neglect the nuclear spin polarization [5, 38] and nuclear spin dynamics, which in principle can take place at submillisecond time scale [39][40][41]. Further, we neglect the anisotropy of the hyperfine interaction [33,42], and assume that the distribution function of the Overhauser field has the form [43,44]:…”
Section: A Modelmentioning
confidence: 99%
“…As a result, the electron g factor equals to 2 in all the QDs. Moreover, since the hyperfine interaction is dominated by the contact interaction with the As nuclei [33], the composition variations in (In,Al)As do not lead to variations of ∆ B . Further, in experiment we detect the PL in a rather narrow window 1.66 − 1.70 eV, which reduces the variance of QD sizes and, as a result, of B ex and ∆ B .…”
Section: Comparison Between Experiments and Theorymentioning
A novel spin orientation mechanism -dynamic electron spin polarization has been recently suggested in Phys. Rev. Lett. 125, 156801 (2020). It takes place for unpolarized optical excitation in weak magnetic fields of the order of a few millitesla. In this paper we demonstrate experimentally and theoretically that the dynamic electron spin polarization degree changes sign as a function of time, strength of the applied magnetic field and its direction. The studies are performed on indirect band-gap (In,Al)As/AlAs quantum dots and their results are explained in the framework of a theoretical model developed for our experimental setting.
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